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To reveal the distribution of atmospheric tritium water (HTO) vapor and provide a baseline for tritium pollution control, a subnational survey was conducted in mainland China. As the largest study on HTO vapor in China that has ever been formally reported, this study provides a macroimpression of the atmospheric HTO specific activity from March 2017 to March 2018. A total of 102 passive samplers were deployed at 34 sites in 30 provinces to determine the seasonal and spatial distributions of HTO vapor. In general, the HTO specific activity in the atmosphere ranged from lower than the minimum detectable activity (0.18 Bq·L–1) to 5.5 Bq·L–1. Spatially, the specific activity of HTO was positively correlated to the latitude and the distance to proximal coastline. Seasonally, significantly higher HTO specific activities were observed in spring and relatively lower in summer. Based on correlation analysis, the atmospheric HTO distributions were considered to be the consequence of combined factors of the stratospheric–tropospheric net mass flux, the distance from the tropopause to the ground, the fraction of air mass that originated from ocean re-evaporation and long-distance transport from high-latitude continents.

In Fukushima, government-led decontamination reduced radiation risk and recovered 137Cs-contaminated soil, yet its long-term downstream impacts remain unclear. Here we provide the comprehensive decontamination impact assessment from 2013 to 2018 using governmental decontamination data, high-resolution satellite images and concurrent river monitoring results. We find that regional erosion potential intensified during decontamination (2013–2016) but decreased in the subsequent revegetation stage. Compared with 2013, suspended sediment at the 1-year-flood discharge increased by 237.1% in 2016. A mixing model suggests that the gradually increasing sediment from decontaminated regions caused a rapid particulate 137Cs decline, whereas no significant changes in downstream discharge-normalized 137Cs flux were observed after decontamination. Our findings demonstrate that upstream decontamination caused persistently excessive suspended sediment loads downstream, though with reduced 137Cs concentration, and that rapid vegetation recovery can shorten the duration of such unsustainable impacts. Future upstream remediation should thus consider pre-assessing local natural restoration and preparing appropriate revegetation measures in remediated regions for downstream sustainability.

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