Atmospheric gas discharge is very likely to constrict into filaments and diffuse plasma formation is inefficient in most cases. Developing cost-efficient atmospheric diffuse plasma devices represents a significant challenge for high performance in biomedical decontamination and material processing. Here, we propose an alternative roadmap to produce a diffuse argon plasma jet by expanding and quenching the existing filamentary discharge at the initial or middle stage of streamer development. Possible mechanisms are summarized. With the gas flow velocity comparable to the ion drift one, enhancing ambipolar diffusion near the edge of the positive-streamer channel promotes the radial diffusion of newly-produced electrons, realizing the radial expansion of channel. Weakening electric field in front of the streamer head through head expansion and field offset, prevents the further development of streamer, leading to a positive-pseudo-streamer discharge. Reducing electric field in front of the negative-streamer head through ion compensation, impedes the initial growth of streamer, resulting in a negative pulseless glow discharge. The positive-pseudo-streamer and negative pulseless glow discharges function together to form the diffuse plasma jet.
A two-dimensional fluid model was used to investigate the characteristics of a multiple-current-pulse dielectric barrier discharge (DBD) equipped with ring electrodes in helium at atmospheric pressure. The simulation results show that the discharge at peak moment follows the Townsend mode in the DBD with two current pulses in each half cycle. However, when there are three or four current pulses in each half cycle, the discharge mode at the first current peak transforms to the glow mode. Additionally, for the first and third current pulse, the breakdown first occurs in the radial center of the ring electrodes. But for the discharge in the second and fourth current pulse, it ignites from the periphery of the ring electrodes. Moreover, the discharge structure, i.e., the radial spatial distributions of current density, electron density, and electric field at peak moments, shows a feature of alternation between (1) higher current density, electron density, and electric field locating in the radial center of ring electrodes (center-advantage) and (2) higher current density, electron density, and electric field locating in the periphery of ring electrodes (periphery-advantage). This behavior is attributed to the fact that non-uniform surface charge accumulation during the previous discharge has different effects on the electric field in the gas gap in the subsequent discharge.
Developing cost‐efficient large‐scale uniform plasma jets represents a significant challenge for high performance in material processing and plasma medicine. Here, a V–I characteristic modulation approach is proposed to reduce the discharge power and increase the plasma scale and chemical activity in non‐self‐sustained atmospheric direct‐current discharges. The electric field in discharge space is optimized to fundamentally empower simultaneously initiating all discharge cells far below Townsend breakdown potential and stably sustaining each plasma jet at low voltage. These strategies create a crucial step to fabricating a flexible and compact low‐power large‐scale uniform laminar plasma jet array (LPJA) with high activity in cheap argon. The mechanisms behind the discharge enhancement are revealed by combining V–I characteristic examination and a modulation model. Compared with conventional arrays, this LPJA possesses the widest size (90 mm) and raises its uniformity from 30% to 97%. Comparing different discharge modes shows that the LPJA scale is surprisingly increased nearly by 4 times with the discharge power reduced from 7.4 to 4.8 W. The methodology provides a highly cost‐efficient roadmap to break through the bottleneck of restricting low‐power discharge, large‐gap discharge, large‐scale discharge, parallel‐multi‐electrode discharge, and uniform discharge together. This advance will meet the urgent need for various plasma applications.
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