Whether quantum physics is universally valid is an open question with far-reaching implications. Intense research is therefore invested into testing the quantum superposition principle with ever heavier and more complex objects. Here we propose a radically new, experimentally viable route towards studies at the quantum-to-classical borderline by probing the orientational quantum revivals of a nanoscale rigid rotor. The proposed interference experiment testifies a macroscopic superposition of all possible orientations. It requires no diffraction grating, uses only a single levitated particle, and works with moderate motional temperatures under realistic environmental conditions. The first exploitation of quantum rotations of a massive object opens the door to new tests of quantum physics with submicron particles and to quantum gyroscopic torque sensors, holding the potential to improve state-of-the-art devices by many orders of magnitude.

Motivated by trapping and cooling experiments with non-spherical nanoparticles, we discuss how their combined rotational and translational quantum state is affected by the interaction with a gaseous environment. Based on the quantum master equation in terms of orientation-dependent scattering amplitudes, we evaluate the localization rate for gas collisions off an anisotropic van der Waals-type potential and for photon scattering off an anisotropic dielectric. We also show how pure angular momentum diffusion arises from these open quantum dynamics in the limit of weak anisotropies.

We show how to describe the diffusion of the quantized angular momentum vector of an arbitrarily shaped rigid rotor as induced by its collisional interaction with an environment. We present the general form of the Lindblad-type master equation and relate it to the orientational decoherence of an asymmetric nanoparticle in the limit of small anisotropies. The corresponding diffusion coefficients are derived for gas particles scattering off large molecules and for ambient photons scattering off dielectric particles, using the elastic scattering amplitudes.The first term accounts for the free dynamics, the second part describes the effect of the environment. It follows from equation (2), similar to the derivation of the Fokker-Planck equation [27, 29], thatNote that the use of canonical momenta instead of J would render the free evolution in (4) phase space volume preserving, but it would complicate considerably the diffusive part (5).In order to observe that equation (5) indeed describes angular momentum diffusion, we note that the expectation value of J remains constant while its second moment increases linearly with time, J J J 0 and 2 D . 6 t t

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