The reaction network in the neutron-deficient part of the nuclear chart around A ≈ 100 contains several nuclei of importance to astrophysical processes, such as the p–process. This work reports on the results from recent experimental studies of the radiative proton–capture reactions 112,114Cd(p, γ)113,115 In. Experimental cross sections for the reactions have been measured for proton beam energies residing inside the respective Gamow windows for each reaction, using isotopically enriched 112Cd and 114Cd targets. Two different techniques, the in–beam γ–ray spectroscopy and the activation method have been implemented, where the latter is considered mandatory to account for the presence of low–lying isomers in 113In (E ≈ 392 keV, t1/2 ≈ 100 min), and 115In (E ≈ 336 keV, t1/2 ≈ 4.5 h). Following the measurement of the cross sections, the astrophysical S factors have been subsequently
About 35 nuclides which lie on the neutron deficient side of the isotopic chart cannot be created by the two basic nucleosynthetic processes, the sand the rprocess. Due to scarce experimental data and the vast complexity of the reaction network involved, cross sections and reactions are estimated theoretically, using the Hauser–Feshbach statistical model. In the present work, theoretical calculations of cross sections of radiative α-capture reactions on the neutron–deficient Erbium and Xenon isotopes are presented in an attempt to make predictions inside the astrophysically relevant energy window (Gamow). The particular reactions are predicted to be sensitive branchings in the γprocess path.The most recent versions of TALYS (v1.9) and Fresco codes were employed for all calculations, initially focusing on investigating the influence of the default eight (8) α–nucleus optical potential models of TALYS on reaction cross sections. The theoretical results of both codes are compared and for the reactions where experimental data exist in literature, the optical model parameters were adjusted appropriately to best describe the data and were subsequently used for estimating (α,γ) reaction cross sections. Predictions for the (α,n) reaction channels have also been calculated and studied.
A mobile γ–ray spectrometer (AMESOS) has been developed using a 3”×3” NaI(Tl) detector, a custom–made mounting holder, and portable electronics to perform in situ measurements of radioactivity. The spectrometer was calibrated using standard point sources and its absolute efficiency was determined. As a field test operation, AMESOS was deployed on the premises of the University of Athens Zografou campus focusing on estimating the NORM levels. Data were analyzed and used to create radiological maps for the metropolitan UoA campus for the first time. Besides natural radioactivity levels, trace concentrations of 137Cs were also detected, attributed to the Chernobyl fallout in Greece. An overall steady performance of the spectrometer was observed throughout the field operation. AMESOS is ready to be deployed for in situ studies of environmental radioactivity and radwaste management.
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