The integrated-path differential-absorption lidar CHARM-F (CO and CH Remote Monitoring-Flugzeug) was developed for the simultaneous measurement of the greenhouse gases CO and CH onboard the German research aircraft HALO (High Altitude and Long Range Research Aircraft). The purpose is to derive the weighted, column-averaged dry-air mixing ratios of the two gases with high precision and accuracy between aircraft and ground or cloud tops. This paper presents the first measurements, performed in the spring of 2015, and shows performance analyses as well as the methodology for the quantification of strong point sources applied on example cases. A measurement precision of below 0.5% for 20 km averages was found. However, individual measurements still show deviations of the absolute mixing ratios compared to corresponding data from in situ profiles. The detailed analysis of the methane point source emission rate yields plausible results (26±3  m/min or 9.2±1.15  kt CH yr), which is in good agreement with reported numbers. In terms of CO, a power plant emission could be identified and analyzed.

Carbon dioxide (CO2) and methane (CH4) are the most important of the greenhouse gases that are directly influenced by human activities. The Integrated Path Differential Absorption (IPDA) lidar technique using hard target reflection in the near IR (1.57µm and 1.64µm) to measure the column-averaged dry air mixing ratio of CO2 and CH4 with high precision and low bias has the potential to deliver measurements from space and air that are needed to understand the sources and sinks of these greenhouse gases. CO2 and CH4 IPDA require tunable laser sources at 1.57 µm and 1.64 µm that coincide with appropriate absorption lines of these species having high pulse energy and average power as well as excellent spectral and spatial properties.Within this study we have realized more than 50mJ of pulse energy in the near IR coincident with appropriate absorption lines using an injection-seeded optical parametric oscillator-amplifier system pumped at 100 Hz. At the same time this device showed excellent spectral and spatial properties. Bandwidths of less than 100 MHz with a high degree of spectral purity (> 99.9 %) have been achieved. The frequency stability was likewise excellent. The M 2 -factor was better than 2.3.Owing to these outstanding properties optical parametric devices are currently under investigation for the CH4 lidar instrument on the projected French-German climate satellite MERLIN. A similar device is under development at DLR for the lidar demonstrator CHARM-F which will enable the simultaneous measurement of CO2 and CH4 from an airborne platform.

We report on the development of a pulsed neodymium-doped yttrium aluminum garnet (Nd:YAG) laser operating at a 1116 nm wavelength. Because the third harmonic is within a few gigahertz of the 372 nm absorption line of iron, this laser system represents an alternative to alexandrite lasers commonly used in iron fluorescence lidars. With our prototype, we achieved a 0.5 W at 372 nm wavelength and a 100 Hz pulse repetition frequency. As a proof of concept, we show iron density measurements, which have been acquired using the novel lidar transmitter.

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For the CO 2 and CH 4 IPDA lidar CHARM-F two single frequency Nd:YAG based MOPA systems were developed. Both lasers are used for OPO/OPA-pumping in order to generate laser radiation at 1645 nm for CH 4 detection and 1572 nm for CO 2 detection. By the use of a Q-switched, injection seeded and actively length-stabilized oscillator and a one-stage INNOSLAB amplifier about 85 mJ pulse energy could be generated for the CH 4 system. For the CO 2 system the energy was boosted in second INNOSLAB-stage to about 150 mJ. Both lasers emit laser pulses of about 30 ns pulse duration at a repetition rate of 100 Hz.