Odin is a 250 kg class satellite built in co-operation between Sweden, Canada, France, and Finland and launched in February 2001. It carries two instruments: a 4-band sub-millimetre radiometer used for both astronomy and atmospheric science and an optical spectrometer and infrared imaging system for purely atmospheric observations. As part of the joint mission Odin will observe the atmospheric limb for 50% of the observation time producing profiles of many species of interest in the middle atmosphere with a vertical resolution of 1–2 km. These species include, among others, ozone, nitrogen dioxide, chlorine monoxide, nitric acid, water vapour, and nitrous oxide. An overview of the mission and the planned measurements is given. PACS Nos.: 42.68Mj, 94.10Dy, 95.55Fw

The optical spectrograph and infrared imager system (OSIRIS) on board the Odin spacecraft is designed to retrieve altitude profiles of terrestrial atmospheric minor species by observing limb-radiance profiles. The grating optical spectrograph (OS) obtains spectra of scattered sunlight over the range 280-800 nm with a spectral resolution of approximately 1 nm. The Odin spacecraft performs a repetitive vertical limb scan to sweep the OS 1 km vertical field of view over selected altitude ranges from approximately 10 to 100 km. The terrestrial absorption features that are superimposed on the scattered solar spectrum are monitored to derive the minor species altitude profiles. The spectrograph also detects the airglow, which can be used to study the mesosphere and lower thermosphere. The other part of OSIRIS is a three-channel infrared imager (IRI) that uses linear array detectors to image the vertical limb radiance over an altitude range of approximately 100 km. The IRI observes both scattered sunlight and the airglow emissions from the oxygen infrared atmospheric band at 1.27 µm and the OH (3-1) Meinel band at 1.53 µm. A tomographic inversion technique is used with a series of these vertical images to derive the two-dimensional distribution of the emissions within the orbit plane.Résumé : Le système de spectrographie optique et d'imagerie infrarouge (OSIRIS) à bord du satellite Odin est conçu pour enregistrer les profils en altitude des éléments mineurs de l'atmosphère en observant les profils de radiance du limbe. Le spectrographe optique à réseau (OS) obtient les spectres de la lumière solaire diffusée sur le domaine entre 280-800 nm, avec une résolution spatiale approximative de 1 nm. Le satellite Odin balaye verticalement le limbe de façon répétée, de telle sorte que l'ouverture verticale de 1 km du OS parcoure les domaines voulus entre 10 et 100 km. Nous analysons les spectres solaires diffusés en superposition avec les caractéristiques terrestres d'absorption, afin de déterminer les profils en altitude des éléments mineurs de l'atmosphère. Le spectrographe détecte aussi la luminescence nocturne atmosphérique qui peut être utilisé pour étudier la mésosphère et la thermosphère. L'autre partie d'OSIRIS est un imageur infrarouge (IRI) à trois canaux qui utilise une banque linéaire de détecteurs pour imager la radiance du limbe sur un domaine d'altitude d'approximativement 100 km. L'IRI observe à la fois la lumière solaire diffusée et les émissions de luminescence nocturne atmospérique provenant de la bande infrarouge de l'oxygène atmosphérique à 1.27 µm et la bande de Meinel de l'OH (3-1) à 1.53 µm. Nous utilisons une technique d'inversion tomographique avec une série de ces images verticales pour obtenir la distribution bidimensionnelle des émissions à l'intérieur de l'orbite.[Traduit par la Rédaction] Can.

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Abstract. A correct and reliable forecast of volcanic plume dispersion is vital for aviation safety. This can only be achieved by representing all responsible physical and chemical processes (sources, sinks, and interactions) in the forecast models. The representation of the sources has been enhanced over the last decade, while the sinks and interactions have received less attention. In particular, aerosol dynamic processes and aerosol–radiation interaction are neglected so far. Here we address this gap by further developing the ICON-ART (ICOsahedral Nonhydrostatic – Aerosols and Reactive Trace gases) global modeling system to account for these processes. We use this extended model for the simulation of volcanic aerosol dispersion after the Raikoke eruption in June 2019. Additionally, we validate the simulation results with measurements from AHI (Advanced Himawari Imager), CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization), and OMPS-LP (Ozone Mapping and Profiling Suite-Limb Profiler). Our results show that around 50 % of very fine volcanic ash mass (particles with diameter d<30 µm) is removed due to particle growth and aging. Furthermore, the maximum volcanic cloud top height rises more than 6 km over the course of 4 d after the eruption due to aerosol–radiation interaction. This is the first direct evidence that shows how cumulative effects of aerosol dynamics and aerosol–radiation interaction lead to a more precise forecast of very fine ash lifetime in volcanic clouds.

[1] Vertical profiles of stratospheric bromine monoxide (BrO) in the 15-30 km range are retrieved from SCIAMACHY limb scatter data over the globe. First validation comparisons with the balloon-borne SAOZ-BrO and LPMA/DOAS instruments indicate retrieval biases of $20% or less. Propagated spectral fitting uncertainties lead to a precision approaching $25% on a 2 km grid at 25 km. This worsens at higher altitudes because of reduced signal and at lower altitudes because of the reduced penetrability of the atmosphere. In terms of volume mixing ratio (VMR), the single profile precision increases from $4 pptv at 17 km to $8 pptv at 27 km. Repeatability, an alternative indicator of precision, is 2-3 pptv for SCIAMACHY retrievals and independent of altitude. The BrO stratospheric number density peak generally lies 5 ± 2 km above the tropopause. In the tropics, the stratospheric BrO VMR generally increases with increasing altitude. The observed stratospheric BrO global distribution is generally consistent with previous balloon measurements but does not agree well with results of a model that uses Br y inferred only from the observed breakdown of long-lived bromoalkanes (i.e., methyl bromide and halons). We find best agreement with the observed vertical and latitudinal distribution of BrO for model results that include an 8.4 ± 2 pptv contribution to stratospheric Br y , most of which is expected from the breakdown of VSL (very short lived) bromocarbons, in addition to the $16 pptv contribution from longer-lived sources. This suggests that stratospheric Br y exceeds 20 pptv. Profiles of Br y profiles derived from the balloon measurements of BrO also suggest Br y is in excess of 20 pptv, but the uncertainty and variability of these results do not allow us to definitively rule out this concentration. We find typical BrO VMRs of $4 pptv at 15 km in the tropical tropopause layer, suggesting that a significant portion of the bromine from VSL bromoalkane sources may be carried across the tropopause in the form of inorganic decomposition products. We discuss a variety of VSL bromocarbons species that may be contributing to the elevated concentrations of stratospheric BrO.