It has become clear over the last decade that the building industry must rapidly change to meet globally pressing requirements. The strong links between climate change and the environmental impact of architecture mean an urgent necessity for alternative design solutions. In order to propose them in this project, two emergent fabrication techniques were deployed with natural fiber-reinforced polymers (NFRPs), namely tailored fiber placement (TFP) and coreless filament winding (CFW). The approach is explored through the design and prototyping of a stool, as an analogue of the functional and structural performance requirements of an architectural system. TFP and CFW technologies are leveraged for their abilities of strategic material placement to create high-performance differentiated structure and geometry. Flax fibers, in this case, provide a renewable alternative for high-performance yarns, such as carbon, glass, or basalt. The novel contribution of this project is exploring the use of a TFP preform as an embedded fabrication frame for CFW. This eliminates the complex, expensive, and rigid molds that are traditionally associated with composites. Through a bottom-up iterative method, material and structure are explored in an integrative design process. This culminates in a lightweight FlexFlax Stool design (ca. 1 kg), which can carry approximately 80 times its weight, articulated in a new material-based design tectonic.