Exploring the relationship between environmental air quality (EAQ) and climatic conditions on a large scale can help better understand the main distribution characteristics and the mechanisms of EAQ in China, which is significant for the implementation of policies of joint prevention and control of regional air pollution. In this study, we used the concentrations of six conventional air pollutants, i.e., carbon monoxide (CO), sulfur dioxide (SO2), nitrogen dioxide (NO2), fine particulate matter (PM2.5), coarse particulate matter (PM10), and ozone (O3), derived from about 1300 monitoring sites in eastern China (EC) from January 2015 to December 2018. Exploiting the grading concentration limit (GB3095-2012) of various pollutants in China, we also calculated the monthly average air quality index (AQI) in EC. The results show that, generally, the EAQ has improved in all seasons in EC from 2015 to 2018. In particular, the concentrations of conventional air pollutants, such as CO, SO2, and NO2, have been decreasing year by year. However, the concentrations of particulate matter, such as PM2.5 and PM10, have changed little, and the O3 concentration increased from 2015 to 2018. Empirical mode decomposition (EOF) was used to analyze the major patterns of AQI in EC. The first mode (EOF1) was characterized by a uniform structure in AQI over EC. These phenomena are due to the precipitation variability associated with the East Asian summer monsoon (EASM), referred to as the “summer–winter” pattern. The second EOF mode (EOF2) showed that the AQI over EC is a north–south dipole pattern, which is bound by the Qinling Mountains and Huaihe River (about 35° N). The EOF2 is mainly caused by seasonal variations of the mixed concentration of PM2.5 and O3. Associated with EOF2, the Mongolia–Siberian High influences the AQI variation over northern EC by dominating the low-level winds (10 m and 850 hPa) in autumn and winter, and precipitation affects the AQI variation over southern EC in spring and summer.
The last millennium (LM, 1000-1850 AD) is crucial for studying historical climate change on decadal to multidecadal timescales. The summer surface air temperature (SAT) evolutions on regional scales (e.g. over China) are more uncertain than the globe/Northern Hemisphere, especially in response to external forcing factors and internal climate variability. Here, we provide onesignal (full-forcing) fingerprints of summer SAT in China derived from three large ensemble model archives with a multi-proxy reconstruction during the LM, Little Ice Age (LIA, 1451-1850 AD), and Medieval Climate Anomaly (MCA, 1000-1250 AD), respectively. Our results show that (a) SATs in the northeast, southeast, northwest, and Tibetan Plateau (TP) regions of China show evident decreasing trends during the LM. External forcing response from all model archives agrees with the regional SAT reconstruction but underestimates variability in northwest China at the multidecadal timescale. (b) During the LIA, the summer regional SAT exhibits a cold condition in the reconstruction and simulations, especially in the northeast and northwest regions of China. External forcing responses in most model archives are the dominant factor on multidecadal SAT evolutions in the southeast, northeast, and TP regions of China and decadal SAT evolutions in northwest China. (c) During the MCA, detection and attribution of SAT shows that internal climate variability dominates in southeast, northeast, and TP regions of China, but external forcing dominates in northwest China at decadal to multidecadal timescales. These results contribute to a better understanding of the causes and mechanisms of regional climate change.
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