Abstract. The impact of aerosols on cloud properties is one of the largest uncertainties in the anthropogenic radiative forcing of the climate. Significant progress has been made in constraining this forcing using observations, but uncertainty remains, particularly in the magnitude of cloud rapid adjustments to aerosol perturbations. Cloud liquid water path (LWP) is the leading control on liquid-cloud albedo, making it important to observationally constrain the aerosol impact on LWP. Previous modelling and observational studies have shown that multiple processes play a role in determining the LWP response to aerosol perturbations, but that the aerosol effect can be difficult to isolate. Following previous studies using mediating variables, this work investigates use of the relationship between cloud droplet number concentration (Nd) and LWP for constraining the role of aerosols. Using joint-probability histograms to account for the non-linear relationship, this work finds a relationship that is broadly consistent with previous studies. There is significant geographical variation in the relationship, partly due to role of meteorological factors (particularly relative humidity). The Nd–LWP relationship is negative in the majority of regions, suggesting that aerosol-induced LWP reductions could offset a significant fraction of the instantaneous radiative forcing from aerosol–cloud interactions (RFaci). However, variations in the Nd–LWP relationship in response to volcanic and shipping aerosol perturbations indicate that the Nd–LWP relationship overestimates the causal Nd impact on LWP due to the role of confounding factors. The weaker LWP reduction implied by these “natural experiments” means that this work provides an upper bound to the radiative forcing from aerosol-induced changes in the LWP.

Abstract. A technique is presented that uses attenuated backscatter profiles from the CALIOP satellite lidar to estimate cloud base heights of lower-troposphere liquid clouds (cloud base height below approximately 3 km). Even when clouds are thick enough to attenuate the lidar beam (optical thickness τ≳5), the technique provides cloud base heights by treating the cloud base height of nearby thinner clouds as representative of the surrounding cloud field. Using ground-based ceilometer data, uncertainty estimates for the cloud base height product at retrieval resolution are derived as a function of various properties of the CALIOP lidar profiles. Evaluation of the predicted cloud base heights and their predicted uncertainty using a second statistically independent ceilometer dataset shows that cloud base heights and uncertainties are biased by less than 10 %. Geographic distributions of cloud base height and its uncertainty are presented. In some regions, the uncertainty is found to be substantially smaller than the 480 m uncertainty assumed in the A-Train surface downwelling longwave estimate, potentially permitting the most uncertain of the radiative fluxes in the climate system to be better constrained. The cloud base dataset is available at https://doi.org/10.1594/WDCC/CBASE.

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<p><strong>Abstract.</strong> The impact of aerosols on cloud properties is one of the largest uncertainties in the anthropogenic radiative forcing of the climate. In recent years, significant progress has been made in constraining this forcing using observations, but uncertainty still remains, particularly in the adjustments of cloud properties to aerosol perturbations. Cloud liquid water path (LWP) is the leading control on liquid-cloud albedo, making it important to observationally constrain the aerosol impact LWP.</p> <p> Previous modelling and observational studies have shown that multiple processes play a role in determining the LWP response to aerosol perturbations, but that the aerosol effect can be difficult to isolate. Following previous studies using mediating variables, this work investigates use of the relationship between cloud droplet number concentration (N<sub><i>d</i></sub>) and LWP for constraining the role of aerosols. Using joint probability histograms to account for the non-linear relationship, this work finds a relationship that is broadly consistent with previous studies. There is significant geographical variation in the relationship, partly due to role of meteorological factors (particularly relative humidity) in the relationship. However, the N<sub><i>d</i></sub>-LWP relationship is negative in the majority of regions, suggesting that aerosol induced LWP reductions could offset a significant fraction of the radiative forcing from aerosol-cloud interactions (RFaci).</p> <p> However, variations in the N<sub><i>d</i></sub>-LWP relationship in response to volcanic and shipping aerosol perturbations indicate that the N<sub><i>d</i></sub>-LWP relationship overestimates the N<sub><i>d</i></sub> impact on LWP. As such, the estimate of LWP changes due to aerosol in this work provides an upper bound to the radiative forcing from aerosol-induced changes in the LWP.</p>

Clouds are highly variable in time and space, affecting climate sensitivity and climate change. To study and distinguish the different influences of clouds on the climate system, it is useful to separate clouds into individual cloud regimes. In this work we present a new cloud classification for liquid water clouds at cloud scale defined using cloud parameters retrieved from combined satellite measurements from CloudSat and CALIPSO. The idea is that cloud heterogeneity is a measure that allows us to distinguish cumuliform and stratiform clouds, and cloud-base height is a measure to distinguish cloud altitude. The approach makes use of a newly developed cloud-base height retrieval. Using three cloud-base height intervals and two intervals of cloud-top variability as an inhomogeneity parameter provides six new liquid cloud classes. The results show a smooth transition between marine and continental clouds as well as between stratiform and cumuliform clouds in different latitudes at the high spatial resolution of about 20 km. Analysing the micro-and macrophysical cloud parameters from collocated combined MODIS, CloudSat and CALIPSO retrievals shows distinct characteristics for each cloud regime that are in agreement with expectation and literature. This demonstrates the usefulness of the classification.