The unconventional normal-state properties of the cuprates are often discussed in terms of emergent electronic order that onsets below a putative critical doping of xc ≈ 0.19. Charge density wave (CDW) correlations represent one such order; however, experimental evidence for such order generally spans a limited range of doping that falls short of the critical value xc, leading to questions regarding its essential relevance. Here, we use X-ray diffraction to demonstrate that CDW correlations in La2−xSrxCuO4 persist up to a doping of at least x = 0.21. The correlations show strong changes through the superconducting transition, but no obvious discontinuity through xc ≈ 0.19, despite changes in Fermi surface topology and electronic transport at this doping. These results demonstrate the interaction between CDWs and superconductivity even in overdoped cuprates and prompt a reconsideration of the role of CDW correlations in the high-temperature cuprate phase diagram.
The recent discovery of the topologically protected surface states in the β-phase of PdBi2 has reignited the research interest in this class of superconductors. Here, we show results of our muon spin relaxation and rotation (µSR) measurements carried out to investigate the superconducting and magnetic properties and the topological effect in the superconducting ground state of β-PdBi2. Zero-field µSR data reveal that no sizeable spontaneous magnetization arises with the onset of superconductivity implying that the time reversal symmetry is preserved in the superconducting state of β-PdBi2. Further, a strong diamagnetic shift of the applied field has been observed in the transverse-field (TF) µSR experiments, indicating that any triplet-pairing channel, if present, does not dominate the superconducting condensate. Using TF-µSR, we estimate that the magnetic penetration depth λ = 263(10) nm at zero temperature. The nature of λ(T ) provides evidence for the existence of a nodeless single s-wave type isotropic energy gap of 0.78(1) meV at zero temperature. Our results further suggest that the topologically protected surface states have no effect on the bulk of the superconductor.
The discovery of superconductivity in a d 9−δ nickelate has inspired disparate theoretical perspectives regarding the essential physics of this class of materials. A key issue is the magnitude of the magnetic superexchange, which relates to whether cuprate-like high-temperature nickelate superconductivity could be realized. We address this question using Ni L-edge and O K-edge spectroscopy of the reduced d 9−1=3 trilayer nickelates R 4 Ni 3 O 8 (where R ¼ La, Pr) and associated theoretical modeling. A magnon energy scale of ∼80 meV resulting from a nearest-neighbor magnetic exchange of J ¼ 69ð4Þ meV is observed, proving that d 9−δ nickelates can host a large superexchange. This value, along with that of the Ni-O hybridization estimated from our O K-edge data, implies that trilayer nickelates represent an intermediate case between the infinite-layer nickelates and the cuprates. Layered nickelates thus provide a route to testing the relevance of superexchange to nickelate superconductivity.
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