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A performance assessment model for multiple barrier packages containing unreprocessed spent fuel has been modified and applied to several package designs. The objective of the study was to develop information to be used in programmatic decision making concerning engineered barrier package design and development. The assessment models "BARIER''^ was developed in previous tasks of the System Study on Engineered Barriers (SSEB). The new version discussed in this report contains a refined and expanded corrosion rate data base which includes pittingj crack growth, and graphitizatlon as well as bulk corrosion. Corrosion rates for oxic and anoxic conditions at each of the two temperature ranges are supplied. Other Improvements Include a rigorous treatment of radionuclide release after package failure which includes resistance of damaged barriers and backfill 5 refined temperature calculations that account for convection and radiatlonj a subroutine to calculate nuclear gamma radiation field at each barrier surface, refined stress calculations with reduced conservatism and various coding improvements to improve running time and core usage. This report also contains discussion of alternative scenarios to the assumed flooded repository as well as the impact of water exclusion backfills. The model was used to assess post repository closure performance for several designs which were all variation of basic designs from the Spend Unreprocessed Fuel (SURF) program. Many designs were found to delay the onset of leaching by at least a few hundreds of years In all geologic media. Long delay times for radionuclide release were found for packages with a few Inches of sorption backfill. Release of uranium, plutonlum, and americium was assessed.

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rf sputtering of ZnO films

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