The superfluid density ρs(T ) ≡ 1/λ 2 (T ) has been measured at 2.64 GHz in highly underdoped YBa2Cu3O6+y, at 37 dopings with Tc between 3 K and 17 K. Within limits set by the transition width ∆Tc ≈ 0.4 K, ρs(T ) shows no evidence of critical fluctuations as T → Tc, with a meanfield-like transition and no indication of vortex unbinding. Instead, we propose that ρs displays the behaviour expected for a quantum phase transition in the (3 + 1)-dimensional XY universality class, with ρs0PACS numbers: 74.72. Bk, 74.25.Nf, 74.25.Bt, 74.25.Ha Current research on high temperature superconductivity focuses on the underdoped cuprates, in a region of the phase diagram where d-wave superconductivity gives way to antiferromagnetism [1]. One proposal for this regime is that at temperatures up to about 100 K above T c , superconductivity persists locally, with long-range phase coherence suppressed by fluctuations in the phase of the superconducting order parameter [2,3,4,5,6,7,8]. Early results showing a linear relation between T c and the superfluid density ρ s (T = 0) [9] provided the original motivation for this point of view, suggesting that T c is low in underdoped materials because the phase stiffness is low. Further support for this idea has come from measurements showing a finite phase stiffness above T c at terahertz frequencies [10], and from experiments that appear to detect the phase-slip voltage of thermally diffusing vortices in the normal state [11]. If the physics of the underdoped cuprates is indeed that of a fluctuating d-wave superconductor there should be a regime where quantum fluctuations come into play as T c falls to zero with decreasing doping. Here we test this idea with a detailed study of the doping dependence of the superfluid density in the vicinity of the critical doping for superconductivity.High homogeneity of T c is particularly difficult to achieve in the underdoped cuprates, where the control parameter is chemical doping and the materials are well away from plateaus or turning points in T c (y). The YBa 2 Cu 3 O 6+y system has two advantages in this doping range: with careful work, there can be sufficient control of doping homogeneity to produce samples with sharp superconducting transitions [12,13]; and the process of CuO-chain ordering can be harnessed to provide continuous tunability of the carrier density in a single sample, with no change in cation disorder [14]. This is possible because the loosely held chain oxygen atoms in these high quality samples remain mobile at room temperature and gradual ordering into CuO-chain structures slowly pulls electrons from the CuO 2 planes, smoothly increasing hole doping over time [15,16]. For this experiment, single crystals of YBa 2 Cu 3 O 6+y were grown in barium zirconate crucibles and have high purity and low defect levels, with cation disorder at the 10 −4 level [17]. A crystal 0.3 mm thick was cut and polished with Al 2 O 3 abrasive into an ellipsoid of revolution about the sample c-axis, 0.35 mm in diameter. The oxygen content of the elli...
The a-b plane microwave surface impedance of a high-quality Bi 2 Sr 2 CaCu 2 O 8 single crystal ͑T c ഠ 93 K͒ has been measured at 14.4, 24.6, and 34.7 GHz. The surface resistance at low temperature is the lowest yet reported, is comparable with the best YBa 2 Cu 3 O 72d data, and has a characteristic v 2 frequency dependence. The change in penetration depth, Dl ab ͑T ͒, has a strong linear term at low temperature which is consistent with a gap with line nodes on the Fermi surface. The real part of the microwave conductivity displays a broad peak at low temperature, similar to that observed in YBa 2 Cu 3 O 72d . [S0031-9007(96)00735-1]
The lower critical field H(c1) for highly underdoped YBa2Cu3O(6+x) with T(c) between 8.9 and 22 K has been determined by measurements of magnetization M(H) curves with applied field parallel to the c axis. H(c1) is linear in temperatures below about 0.6T(c), and H(c1)(0) is proportional to T(1.64+/-0.04)(c), clearly violating the proportionality between rho(s)(0) and T(c). Moreover, the slope -dH(c1)/dT decreases steeply toward zero as T(c) approaches zero, indicating that the effective charge of the quasiparticles vanishes as the doping is decreased toward the insulating phase.
We calculate superfluid density for a dirty d-wave superconductor. The effects of impurity scattering are treated within the self-consistent t-matrix approximation, in weak-coupling BCS theory. Working from a realistic tight-binding parameterization of the Fermi surface, we find a superfluid density that is both correlated with Tc and linear in temperature, in good correspondence with recent experiments on overdoped La2−xSrxCuO4.
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