[1] Mineral aerosols are produced during the erosion of soils by wind and are a common source of particles (dust) in arid and semiarid regions. The size of these particles varies widely from less than 2 μm to larger particles that can exceed 50 μm in diameter. In this study, we present two continuous records of total suspended particle (TSP) concentrations at sites in Mesa Verde and Canyonlands National Parks in Colorado and Utah, USA, respectively, and compare those values to measurements of fine and coarse particle concentrations made from nearby samplers. Average annual concentrations of TSP at Mesa Verde were 90 μg m À3 in 2011 and at Canyonlands were 171 μg m À3 in 2009, 113 μg m À3 in 2010, and 134 μg m À3 in 2011. In comparison, annual concentrations of fine (diameter of 2.5 μm and below) and coarse (2.5-10 μm diameter) particles at these sites were below 10 μg m À3 in all years. The high concentrations of TSP appear to be the result of regional dust storms with elevated concentrations of particles greater than 10 μm in diameter. These conditions regularly occur from spring through fall with 2 week mean TSP periodically in excess of 200 μg m À3 . Measurement of particles on filters indicates that the median particle size varies between approximately 10 μm in winter and 40 μm during the spring. These persistently elevated concentrations of large particles indicate that regional dust emission as dust storms and events are important determinants of air quality in this region.

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Abstract. The deposition of dust has recently increased significantly over some regions of the western US. Here we explore how changes in dust deposition have affected the biogeochemistry of two alpine watersheds in Colorado, US. We first reconstruct recent changes in the mass accumulation rate of sediments and then we use isotopic measurements in conjunction with a Bayesian mixing model to infer that approximately 95 % of the inorganic fraction of lake sediments is derived from dust. Elemental analyses of modern dust indicate that dust is enriched in Ca, Cr, Cu, Mg, Ni, and in one watershed, Fe and P relative to bedrock. The increase in dust deposition combined with its enrichment in certain elements has altered the biogeochemisty of these systems. Both lakes showed an increase in primary productivity as evidenced by a decrease in carbon isotopic discrimination; however, the cause of increased primary productivity varies due to differences in watershed characteristic. The lake in the larger watershed experienced greater atmospheric N loading and less P loading from the bedrock leading to a greater N:P flux ratio. In contrast, the lake in the smaller watershed experienced less atmospheric N loading and greater P loading from the bedrock, leading to a reduced N:P flux ratio. As a result, primary productivity was more constrained by N availability in the smaller watershed. N-limited primary productivity in the smaller watershed was partly ameliorated by an increase in nitrogen fixation as indicated by reduced nitrogen isotopic values in more contemporary sediments. This study illustrates that alpine watersheds are excellent integrators of changes in atmospheric deposition, but that the biogeochemical response of these watersheds may be mediated by their physical (i.e. watershed area) and chemical (i.e. underlying geology) properties.

Decomposition is central to understanding ecosystem carbon exchange and nutrientrelease processes. Unlike mesic ecosystems, which have been extensively studied, xeric landscapes have received little attention; as a result, abiotic soil-respiration regulatory processes are poorly understood in xeric environments. To provide a more complete and quantitative understanding about how abiotic factors influence soil respiration in xeric ecosystems, we conducted soilrespiration and decomposition-cloth measurements in the cold desert of southeast Utah. Our study evaluated when and to what extent soil texture, moisture, temperature, organic carbon, and nitrogen influence soil respiration and examined whether the inverse-texture hypothesis applies to decomposition. Within our study site, the effect of texture on moisture, as described by the inverse texture hypothesis, was evident, but its effect on decomposition was not. Our results show temperature and moisture to be the dominant abiotic controls of soil respiration. Specifically, temporal offsets in temperature and moisture conditions appear to have a strong control on soil respiration, with the highest fluxes occurring in spring when temperature and moisture were favorable. These temporal offsets resulted in decomposition rates that were controlled by soil moisture and temperature thresholds. The highest fluxes of CO 2 occurred when soil temperature was between 10 and 16°C and volumetric soil moisture was greater than 10%. Decomposition-cloth results, which integrate decomposition processes across several months, support the soil-respiration results and further illustrate the seasonal patterns of high respiration rates during spring and low rates during summer and fall. Results from this study suggest that the parameters used to predict soil respiration in mesic ecosystems likely do not apply in cold-desert environments.