With a combination of an elevated temperature for the β-barium borate (BBO) crystal and an elliptical focusing cavity we succeeded in eliminating the degradation in BBO during second harmonic generation into the ultraviolet (UV). We were capable of generating over 600 mW continuous-wave UV light at 257 nm with an off-the-shelf crystal for over 8 h without any sign of degradation. Our results indicate that the degradation is caused by color centers generated by two-photon absorption (TPA) strongly increasing the absorption of the fundamental radiation. While the higher crystal temperature reduces the TPA coefficient and the life time of the color centers, elliptical focusing strongly reduces the peak irradiance of the fundamental and thus its absorption.
Lasing without inversion is a compelling method based on the generation of coherences between atomic levels in order to produce UV radiation. While the proof-of-principle of this scheme has been shown for several decades, so far no radiation at a significant shorter wavelength than the necessary drive fields has been observed. In a recent publication Rein et al. (Phys Rev. A 105 (2022) 023722) have made experimental progress towards this goal. In this paper, we investigate the necessary improvements to their setup and discuss the experimental steps taken to achieve those goals. Specifically, we report on the improvement with respect to the laser sources.
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