Cost management and scalable fabrication without sacrificing
the
purification performance are two critical issues that should be addressed
before the practical commercial application of solar-driven evaporators.
To address this challenge, we report a porous photothermal hydrogel
coating prepared by mixing the raw materials of sawdust (SD), carbon
nanotubes (CNTs), and poly(vinyl alcohol) (PVA), which was applied
to undergo a blading–drying–rehydration process to prepare
the evaporator. In the coating, the crystallized PVA gives the coating
a solid skeleton and the sawdust endows the coating with a loose structure
to sufficiently enhance the water transportation capacity. As a result,
the evaporator coated with the hydrogel coating displays a high water
transport rate and efficient evaporation performance along with excellent
mechanical properties and stability. Water migrates vertically upward
5 cm within 4 minutes. The compressive stress of the rehydrated hydrogel
coating reaches as high as 14.28 MPa under 80% strain. The water evaporation
rate of the hydrogel coating-based evaporator reaches 1.833 kg m–2 h–1 corresponding to an energy
efficiency of 83.29% under 1 sun irradiation. What is more, the hydrogel
coating retains its excellent evaporation performance and stability
after immersion in acid or alkali solution, ultrasound treatment,
and long-time immersion in water. Under outdoor conditions, the water
evaporation rate of the hydrogel coating-based evaporator is about
5.69 times higher than that of pure water. This study proposes a rapid,
cost-effective, and scalable strategy for preparing a high-performance
photothermal hydrogel coating that will find sustainable and practical
application in solar-driven water purification.
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