High-performance
flexible pressure sensors are highly desirable in health monitoring,
robotic tactile, and artificial intelligence. Construction of microstructures
in dielectrics and electrodes is the dominating approach to improving
the performance of capacitive pressure sensors. Herein, we have demonstrated
a novel three-dimensional microconformal graphene electrode for ultrasensitive
and tunable flexible capacitive pressure sensors. Because the fabrication
process is controllable, the morphologies of the graphene that is
perfectly conformal with the electrode are controllable consequently.
Multiscale morphologies ranging from a few nanometers to hundreds
of nanometers, even to tens of micrometers, have been systematically
investigated, and the high-performance capacitive pressure sensor
with high sensitivity (3.19 kPa–1), fast response
(30 ms), ultralow detection limit (1 mg), tunable-sensitivity, high
flexibility, and high stability was obtained. Furthermore, an ultrasensitivity
of 7.68 kPa–1 was successfully achieved via symmetric
double microconformal graphene electrodes. The finite element analysis
indicates that the microstructured graphene electrode can enhance
large deformation and thus effectively improve the sensitivity. Additionally,
the proposed pressure sensors are demonstrated with practical applications
including insect crawling detection, wearable health monitoring, and
force feedback of robot tactile sensing with a sensor array. The microconformal
graphene may provide a new approach to fabricating controllable microstructured
electrodes to enhance the performance of capacitive pressure sensors
and has great potential for innovative applications in wearable health-monitoring
devices, robot tactile systems, and human–machine interface
systems.
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