This review provides an overview of emerging ultrafast synthesis technologies for energy and environmental applications. Representative ultrafast methods include Joule heating, plasma, laser, infrared, microwave, and flame-assisted synthesis, etc.
Recycling of spent lithium-ion batteries is essential
for the sustainable
development of renewable energy technologies, as it promotes resource
reuse and environmental protection. Recycling cathode materials is
particularly important due to their high concentration of strategic
elements. However, traditional recycling methods for cathode materials
are often inefficient due to high energy consumption and prolonged
operation time. Here, we present an efficient, one-step, nondestructive
method for regenerating spent LiCoO2 cathodes within seconds.
This method simultaneously achieves relithiation of the cathode material
and repair of the crystal structure through rapid Joule heating. Compared
to traditional repair methods, this process exhibits low energy consumption
and shortened operation time. After an 8 s repair process, the regenerated
LiCoO2 has a well-defined layered structure and is restored
to its original electrochemical performance, with an initial discharge
capacity of 133.0 mAh/g and good cycling performance. This work represents
a potentially universal approach for the efficient direct regeneration
of cathode materials.
Lithium metal is widely regarded as the "ultimate" anode for energy-dense Li batteries, but its high reactivity and delicate interface make it prone to dendrite formation, limiting its practical use. Inspired by self-assembled monolayers on metal surfaces, we propose a facile yet effective strategy to stabilize Li metal anodes by creating an artificial solid electrolyte interphase (SEI). Our method involves dip-coating Li metal in MPDMS to create an SEI layer that is rich in inorganic components, allowing uniform Li plating/stripping under a low overpotential over 500 cycles in carbonate electrolytes. In comparison, pristine Li metal shows a rapid increase in overpotential after merely 300 cycles, leading to failure soon after. Molecular dynamics simulations demonstrate that this uniform artificial SEI suppresses Li dendrite formation. We further demonstrated its enhanced stability pairing with LiFePO 4 and LiNi 1−x−y Co x Mn y O 2 cathodes, highlighting the proposed strategy as a promising solution for practical Li metal batteries.
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