The front cover artwork is provided by the Steinbock group at Florida State University. The image shows a pseudo‐color micrograph of biomorph bundles (cyan) pushing a resin disk (red/cyan) as well as other, partly helical, structures (green). Biomorphs consist of nanostructured BaCO3 and silica. Read the full text of the Article at 10.1002/syst.202000061.

Biomorphs are polycrystalline assemblies that form when barium, silicate, and carbonate ions react in basic solutions. Their micrometer‐scale morphologies include leaf‐like sheets, helices, and cones, while their nanoscale architecture is based on co‐aligned witherite nanorods. We report a biomorph shape that resembles hair strands that smoothly curl into spirals or twisting fiber ribbons. They can thicken through continuous fractal‐like branching or abrupt events in which fibers split simultaneously. Raman and energy dispersive X‐ray spectroscopy as well as optical polarization microscopy reveal that their composition is very similar to classical biomorphs. They are most abundant in the absence of glass substrates and at high pH values. However, if a glass surface is covered by a thin SU‐8 resin layer, their growth is observed and photolithographically produced SU‐8 posts serve as nucleation sites. The hair‐like structures can detach resin posts from the glass surface and reposition them due to continued growth at the hair‐resin interface. Collisions of growing biomorph sheets with SU‐8 posts result in overgrowth or a sheet‐to‐hair transition.

The Front Cover shows a pseudo‐color representation of an optical micrograph illustrating two key findings: a new type of polycrystalline biomorph (cyan) and its ability to dislodge, push, and flip small resin disks (red/cyan). More information can be found in the Article by Oliver Steinbock and co‐workers.