The metrology of laser-induced damage usually finds a single transition from 0% to 100% damage probability when progressively increasing the laser energy in experiments. We observe that picosecond pulses at 2-µm wavelength focused inside silicon provide a response that strongly deviates from this. Supported by nonlinear propagation simulations and energy flow analyses, we reveal an increased light delocalization for near critical power conditions. This leads to a nonmonotonic evolution of the peak delivered fluence as a function of the incoming pulse of the energy, a situation more complex than the clamping of the intensity until now observed in ultrafast regimes. Compared to femtosecond lasers, our measurements show that picosecond sources lead to reduced thresholds for three-dimensional (3D) writing inside silicon that is highly desirable. However, strong interplays between nonlinear effects persist and should not be ignored for the performance of future technological developments. We illustrate this aspect by carefully retrieving from the study the conditions for a demonstration of 3D data inscription inside a silicon wafer.

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An original architecture of an active fiber allowing a nearly diffraction-limited beam to be produced is demonstrated. The active medium is a double-clad large-mode-area photonic-bandgap fiber consisting of a 10,000 ppm by weight Yb(3+)-doped core surrounded by an alternation of high- and low-index layers constituting a cylindrical photonic crystal. The periodic cladding allows the robust propagation of a approximately 200 microm(2) fundamental mode and efficiently discriminates against the high-order modes. The M(2) parameter was measured to be 1.17. A high-power cw laser was built exhibiting 80% slope efficiency above threshold. The robust propagation allows the fiber to be tightly bent. Weak incidence on the slope efficiency was observed with wounding radii as small as 6 cm.

Very large mode area, active optical fibers with a low high order mode content in the actively doped core region were designed by removing the inner cladding symmetry. The relevance of the numerical approach is demonstrated here by the investigation of a standard air-silica Large Pitch Fiber, used as a reference. A detailed study of all-solid structures is also performed. Finally, we propose new kinds of geometry for 50 μm core, all-solid microstructured fibers enabling a robust singlemode laser emission from 400 nm to 2200 nm.

The enhancement and control of non-linear phenomena at a nanometer scale has a wide range of applications in science and in industry. Among these phenomena, high-harmonic generation in solids is a recent focus of research to realize next generation petahertz optoelectronic devices or compact all solid state EUV sources. Here, we report on the realization of the first nanoscale high harmonic source. The strong field regime is reached by confining the electric field from a few nanojoules femtosecond laser in a single 3D semiconductor waveguide. We reveal a strong competition between enhancement of coherent harmonics and incoherent fluorescence favored by excitonic processes. However, far from the band edge, clear enhancement of the harmonic emission is reported with a robust sustainability offering a compact nanosource for applications. We illustrate the potential of our harmonic nano-device by performing a coherent diffractive imaging experiment. Ultra-compact UV/X-ray nanoprobes are foreseen to have other applications such as petahertz electronics, nano-tomography or nano-medicine.