Metasurfaces constitute a powerful approach to generate and control light by engineering optical material properties at the subwavelength scale. Recently, this concept was applied to manipulate free-electron radiation phenomena, rendering versatile light sources with unique functionalities. In this Letter, we experimentally demonstrate spectral and angular control over coherent light emission by metasurfaces that interact with freeelectrons under grazing incidence. Specifically, we study metalenses based on chirped metagratings that simultaneously emit and shape Smith−Purcell radiation in the visible and near-infrared spectral regime. In good agreement with theory, we observe the far-field signatures of strongly convergent and divergent cylindrical radiation wavefronts using in situ hyperspectral angle-resolved light detection in a scanning electron microscope. Furthermore, we theoretically explore simultaneous control over the polarization and wavefront of Smith−Purcell radiation via a split-ring-resonator metasurface, enabling tunable operation by spatially selective mode excitation at nanometer resolution. Our work highlights the potential of merging metasurfaces with free-electron excitations for versatile and highly tunable radiation sources in wide-ranging spectral regimes.

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Electron beam shaping by sculpted thin films relies on electron–matter interactions and the wave nature of electrons. It can be used to study physical phenomena of special electron beams and to develop technological applications in electron microscopy that offer new and improved measurement techniques and increased resolution in different imaging modes. In this Perspective, we review recent applications of sculpted thin films for electron orbital angular momentum sorting, improvements in phase contrast transmission electron microscopy, and aberration correction. For the latter, we also present new results of our work toward correction of the spherical aberration of Lorentz scanning transmission electron microscopes and suggest a method to correct chromatic aberration using thin films. This review provides practical insight for researchers in the field and motivates future progress in electron microscopy.

We demonstrate focused emission of visible and near-infrared Smith-Purcell radiation by a free-electron-driven metasurface lens emitter. Our findings pave the way for free-electron light sources focusing at wavelengths lacking efficient optics.