Gamma-ray spectral data were collected from sensors mounted to traffic signals around Northern Virginia. The data were collected over a span of approximately fifteen months. A subset of the data were analyzed manually and subsequently used to train machine-learning models to facilitate the evaluation of the remaining 50k anomalous events identified in the dataset. We describe the analysis approach used here and discuss the results in terms of radioisotope classes and frequency patterns over day-of-week and time-of-day spans. Data from this work has been archived and is available for future and ongoing research applications.