Abstract. Air quality degradation is a major issue in the large conurbations on the shore of the Gulf of Guinea. We present for the first time PM 2.5 time series collected in Cotonou, Benin, and Abidjan, Côte d'Ivoire, from February 2015 to March 2017. Measurements were performed in the vicinity of major combustion aerosol sources: Cotonou/traffic (CT), Abidjan/traffic (AT), Abidjan/landfill (AL) and Abidjan/domestic fires (ADF). We report the weekly PM 2.5 mass and carbonaceous content as elemental (EC) and organic (OC) carbon concentrations. We also measure the aerosol optical depth (AOD) and the Ångström exponent in both cities. The average PM 2.5 mass concentrations were 32 ± 32, 32 ± 24 and 28 ± 19 µg m −3 at traffic sites CT and AT and landfill site AL, respectively. The domestic fire site shows a concentration of 145 ± 69 µg m −3 due to the contribution of smoking and roasting activities. The highest OC and EC concentrations were also measured at ADF at 71 ± 29 and 15 ± 9 µg m −3 , respectively, while the other sites present OC concentration between 8 and 12 µg m −3 and EC concentrations between 2 and 7 µg m −3 . The OC / EC ratio is 4.3 at CT and 2.0 at AT. This difference highlights the influence of two-wheel vehicles using gasoline in Cotonou compared to that of four-wheel vehicles using diesel fuel in Abidjan. AOD was rather similar in both cities, with a mean value of 0.58 in Cotonou and of 0.68 in Abidjan. The seasonal cycle is dominated by the large increase in surface mass concentration and AOD during the long dry season (December-February) as expected due to mineral dust advection and biomass burning activities. The lowest concentrations are observed during the short dry season (August-September) due to an increase in surface wind speed leading to a better ventilation. On the other hand, the high PM 2.5 / AOD ratio in the short wet season (October-November) indicates the stagnation of local pollution.
Abstract. A number of campaigns have been carried out to establish the emission factors of pollutants from fuel combustion in West Africa, as part of work package 2 (“Air Pollution and Health”) of the DACCIWA (Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa) FP7 program. Emission sources considered here include wood (hevea and iroko) and charcoal burning, charcoal making, open trash burning, and vehicle emissions, including trucks, cars, buses and two-wheeled vehicles. Emission factors of total particulate matter (TPM), elemental carbon (EC), primary organic carbon (OC) and volatile organic compounds (VOCs) have been established. In addition, emission factor measurements were performed in combustion chambers in order to reproduce field burning conditions for a tropical hardwood (hevea), and obtain particulate emission factors by size (PM0.25, PM1, PM2.5 and PM10). Particle samples were collected on quartz fiber filters and analyzed using gravimetric method for TPM and thermal methods for EC and OC. The emission factors of 58 VOC species were determined using offline sampling on a sorbent tube. Emission factor results for two species of tropical hardwood burning of EC, OC and TPM are 0.98 ± 0.46 g kg−1 of fuel burned (g kg−1), 11.05 ± 4.55 and 41.12 ± 24.62 g kg−1, respectively. For traffic sources, the highest emission factors among particulate species are found for the two-wheeled vehicles with two-stroke engines (2.74 g kg−1 fuel for EC, 65.11 g kg−1 fuel for OC and 496 g kg−1 fuel for TPM). The largest VOC emissions are observed for two-stroke two-wheeled vehicles, which are up to 3 times higher than emissions from light-duty and heavy-duty vehicles. Isoprene and monoterpenes, which are usually associated with biogenic emissions, are present in almost all anthropogenic sources investigated during this work and could be as significant as aromatic emissions in wood burning (1 g kg−1 fuel). EC is primarily emitted in the ultrafine fraction, with 77 % of the total mass being emitted as particles smaller than 0.25 µm. The particles and VOC emission factors obtained in this study are generally higher than those in the literature whose values are discussed in this paper. This study underlines the important role of in situ measurements in deriving realistic and representative emission factors.
In this study, we investigate changes in temperature and precipitation extremes over West and Central Africa (hereafter, WAF domain) as a function of global mean temperature with a focus on the implications of global warming of 1.5 • C and 2 • C according the Paris Agreement. We applied a scaling approach to capture changes in climate extremes with increase in global mean temperature in several subregions within the WAF domain: Western Sahel, Central Sahel, Eastern Sahel, Guinea Coast and Central Africa including Congo Basin.While there are several uncertainties and large ensemble spread in the projections of temperature and precipitation indices, most models show high-impact changes in climate extremes at subregional scale. At these smaller scales, temperature increases within the WAF domain are projected to be higher than the global mean temperature increase (at 1.5 • C and at 2 • C) and heat waves are expected to be more frequent and of longer duration. The most intense warming is observed over the drier regions of the Sahel, in the central Sahel and particularly in the eastern Sahel, where the precipitation and the soil moisture anomalies have the highest probability of projected increase at a global warming of 1.5 • C. Over the wetter regions of the Guinea Coast and Central Africa, models project a weak change in total precipitation and a decrease of the length of wet spells, while these two regions have the highest increase of heavy rainfall in the WAF domain at a global warming of 1.5 • C. Western Sahel is projected by 80% of the models to experience the strongest drying with a significant increase in the length of dry spells and a decrease in the standardized precipitation evapotranspiration index. This study suggests that the 'dry gets drier, wet gets wetter' paradigm is not valid within the WAF domain.
This study aims to understand and document the occurrence and variability of cloud cover types in West Africa (WA). Investigations are carried out with a 10‐year hourly record of two cloud data products: CERES passive satellite observations and ERA5 reanalysis. The seasonal evolutions of high (HCC), middle (MCC), low (LCC) and total (TCC) cloud cover are examined. Both products agree on the seasonal and spatial occurrence of cloud cover, although CERES presents lower values of cloud fraction than ERA5 which is partly attributed to the inability of the satellite sensor to detect optically thin clouds in the atmosphere. Southern WA is found to be cloudier than other parts of the region in all seasons with mean TCC fractions of 70 and 80% for CERES and ERA5 respectively during the monsoon season. In all seasons, the presence of LCC over large areas of the Sahel/Sahara region is noted in the CERES product. This could be due to a possible misinterpretation of Saharan dust as low clouds which may have thus, caused it to overestimate the occurrences and fractions of LCC over this region. Northern WA is associated with higher frequencies of no cloud occurrence events, unlike the south where cloudless skies are rarely observed. Furthermore, in southern WA, overcast conditions of LCC are observed for a significant number of times (up to 20% of the time during the rainy season in CERES and 40% in ERA5). The climatology of cloud cover presented in this study could be useful for the planning of solar energy projects.
Dust generation and transportation from North Africa are thought to modulate the West African Monsoon (WAM) features. In this study, we investigated the relationship between the Saharan Air Layer located above Atlantic Ocean (OSAL) and WAM features, including Monsoon flow, African Easterly Jet (AEJ) and Tropical Easterly Jet (TEJ) over West Africa using the RegCM4 regional model at 30 km grid resolution. Two sets of experiments with and without dust load were performed between 2007 and 2013 over the simulation domain, encompassing the whole of West Africa and a large part of the adjacent Atlantic Ocean. An intercomparison of the two simulations shows that dust load into the atmosphere greatly influences both the wind and temperature structure at different levels, resulting in the observed changes in the main features of the WAM system during summer. These changes lead to a westward shift with a slight strengthening of AEJ core over tropical Atlantic and weakening of both TEJ and monsoon flux penetration over land. In addition, despite running the RegCM4 with prescribed sea surface temperature, a correlation has been found between Aerosol Optical Depths in OSAL and WAM dynamics suggesting a mechanistic link between dust and WAM well reproduced by RegCM4.
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