We present an exhaustive experimental and theoretical study of the shapes of simple and compound jets formed when one (simple) or two (compound) immiscible liquids are injected into another liquid. The viscosity of the co-flowing external liquid is chosen to vary the characteristic Reynolds number of the outer stream, $Re_{o}$, over a wide range of values. Our slender-body theory in Gordillo et al. (J. Fluid Mech., vol. 738, 2014, pp. 335–357) is extended to predict the shapes of simple jets when $Re_{o}$ is such that $Re_{o}\gg 1$ and also to predict the shapes of compound jets in the case of $Re_{o}\lesssim O(1)$. The validity of our theoretical results, applicable to describe the dynamics of simple or compound jets within an outer carrier fluid in a wide variety of practical situations, is tested using a set-up where the liquids flow from a pressurized chamber towards an extraction tube, finding a very good agreement between the predicted and the observed shapes. Moreover, when $Re_{o}\lesssim O(1)$, and thanks to the fact that the liquid jets produced using our method are highly stretched in the downstream direction, we find that the values of the critical capillary number above which a steady stretched jet is produced, with the capillary number defined here using the outer stream velocity and viscosity, is well below the corresponding critical values characterizing other similar procedures, like flow focusing. This experimental result, which is supported by a spatio-temporal stability analysis in which the axial gradients of the unperturbed solution are retained in the dispersion relation, imply a substantial saving of energy and of the volume of outer liquid necessary to generate a steady capillary jet from which drops are regularly produced. Additionally, making use of continuity arguments and of the fact that drops are formed as a consequence of the growth of a capillary instability, we provide closed expressions for the drop diameters and their production frequencies when the capillary number is above the critical one, in very good agreement with experiments. The simple or double microemulsions generated by the capillary disintegration of the type of simple or compound highly stretched steady jets described here might find applications in biotechnology, pharmacy, cosmetics or materials science.
In this paper we reveal the physics underlaying the conditions needed for the generation of emulsions composed of uniformly sized drops of micrometric or submicrometric diameters when two immiscible streams flow in parallel under the so-called tip streaming regime after Suryo & Basaran (2006). Indeed, when inertial effects in both liquid streams are negligible, the inner to outer flow-rate and viscosity ratios are small enough and the capillary number is above an experimentally determined threshold which is predicted by our theoretical results with small relative errors, a steady micron-sized jet is issued from the apex of a conical drop. Under these conditions, the jet disintegrates into drops with a very well defined mean diameter, giving rise to a monodisperse microemulsion. Here, we demonstrate that the regime in which uniformly-sized drops are produced corresponds to values of the capillary number for which the cone-jet system is globally stable. Interestingly enough, our general stability theory reveals that liquid jets with a cone-jet structure are much more stable than their cylindrical counterparts thanks, mostly, to a capillary stabilization mechanism described here for the first time. Our findings also limit the validity of the type of stability analysis based on the common parallel flow assumption to only those situations in which the liquid jet diameter is almost constant.
We provide a detailed physical description of the bubble formation processes taking place in a type of flow where the liquid pressure gradient can be straightforwardly controlled. The analysis, which is supported by an exhaustive experimental study in which the liquid viscosity is varied by three orders of magnitude, provides closed expressions for both the bubbling frequencies and the bubble diameters. Different equations are obtained depending on the values of the three dimensionless parameters characterizing this physical situation, namely the Weber and Reynolds numbers and the gas to liquid flow rate ratio. Since both the inertia dominated and viscous dominated bubbling regimes are simply described in terms of the local pressure gradient and the flow rate ratio, the same types of ideas can be applied in the design of bubble makers in which the pressure gradients are controlled in completely different ways.
We report experiments in which a flow rate Q i of a fluid with a viscosity µ i discharges into an immiscible liquid of viscosity µ o that flows in parallel with the axis of the injector. When the outer capillary number verifies the conditionwhere U o and σ indicate, respectively, the outer velocity and the interfacial tension coefficient, and if the inner-to-outer velocity ratio is such thatwith R i the inner radius of the injector, a jet is formed with the same type of cone-jet geometry as predicted by the numerical results of Suryo & Basaran (Phys. Fluids, vol. 18, 2006, p. 082102). For extremely low values of the velocity ratio U i /U o , we find that the diameter of the jet emanating from the tip of the cone is so small that drops with sizes below 1 µm can be formed. We also show that, through this simple method, concentrated emulsions composed of micrometre-sized drops with a narrow size distribution can be generated. Moreover, thanks to the information extracted from numerical simulations of boundary-integral type and using the slender-body approximation due to Taylor (Proceedings of the 11th International Congress of Applied Mechanics, Munich, 1964, pp. 790-796), we deduce a third-order, ordinary differential equation that predicts, for arbitrary values of the three dimensionless numbers that control this physical situation, namely, Ca o , µ i /µ o and U i /U o , the shape of the jet and the sizes of the drops generated. Most interestingly, the influence of the geometry of the injector system on the jet shape and drop size enters explicitly into the third-order differential equation through two functions that can be easily calculated numerically. Therefore, our theory can be used as an efficient tool for the design of new emulsification devices.
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