Found unknown radioactive material is often contained in a package so the chemical and physical form of the material itself is unknown, and the detail of the packaging is likewise unknown. Together, these present a significant risk on how to handle the package for destructive examination of its contents. Whether of nefarious origin or the result of less stringent practices of yesteryear the material needs to be properly identified and characterized for appropriate disposition. Results of neutron imaging, neutron diffraction, and delayed neutron analysis as applied to an examination of sealed capsules containing unknown radioactive materials are presented. The results demonstrate that neutron-based non-destructive examination techniques can be employed for inspecting encapsulated radioactive samples to identify the materials, to elucidate the internal physical structure of the radioactive material and encapsulation, and to estimate the mass of fissile and fissionable materials within. This characterization of orphaned radioactive special nuclear material illustrates the potential for these techniques in nuclear forensics investigations.
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