We report on high-resolution differential conductance experiments on nanoscale superconductor-ferromagnet tunnel junctions with ultrathin oxide tunnel barriers. We observe subgap conductance features that are symmetric with respect to bias and shift according to the Zeeman energy with an applied magnetic field. These features can be explained by resonant transport via Andreev bound states induced by spin-active scattering at the interface. From the energy and Zeeman shift of the bound states, both the magnitude and sign of the spin-dependent interfacial phase shifts between spin-up and spin-down electrons can be determined. These results contribute to the microscopic insight into the triplet proximity effect at spin-active interfaces.

We report on nonlocal transport in multiterminal superconductor-ferromagnet structures, which were fabricated by means of e-beam lithography and shadow evaporation techniques. In the presence of a significant Zeeman splitting of the quasiparticle states, we find signatures of spin transport over distances of several μm, exceeding other length scales such as the coherence length, the normal-state spin-diffusion length, and the charge-imbalance length. The relaxation length of the spin signal shows a nearly linear increase with magnetic field, hinting at a freeze-out of relaxation by the Zeeman splitting. We propose that the relaxation length is given by the recombination length of the quasiparticles rather than a renormalized spin-diffusion length.

We report on nonlocal transport in superconductor hybrid structures, with ferromagnetic as well as normal-metal tunnel junctions attached to the superconductor. In the presence of a strong Zeeman splitting of the density of states, both charge and spin imbalance is injected into the superconductor. While previous experiments demonstrated spin injection from ferromagnetic electrodes, we show that spin imbalance is also created for normal-metal injector contacts. Using the combination of ferromagnetic and normal-metal detectors allows us to directly discriminate between charge and spin injection, and demonstrate a complete separation of charge and spin imbalance. The relaxation length of the spin imbalance is of the order of several $\mu$m and is found to increase with a magnetic field, but is independent of temperature. We further discuss possible relaxation mechanisms for the explanation of the spin relaxation length.Comment: 7 pages, 6 figures, RevTe

We explore charge imbalance in mesoscopic normal-metal/superconductor multiterminal structures at very low temperatures. The investigated samples, fabricated by e-beam lithography and shadow evaporation, consist of a superconducting aluminum bar with several copper wires forming tunnel contacts at different distances from each other. We have measured in detail the local and non-local conductance of these structures as a function of the applied bias voltage V, the applied magnetic field B, the temperature T and the contact distance d. From these data the charge-imbalance relaxation length lambda_Q* is derived. The bias-resolved measurements show a transition from dominant elastic scattering close to the energy gap to an inelastic two-stage relaxation at higher bias. We observe a strong suppression of charge imbalance with magnetic field, which can be directly linked to the pair-breaking parameter. In contrast, practically no temperature dependence of the charge-imbalance signal was observed below 0.5 K. These results are relevant for the investigation of other non-local effects such as crossed Andreev reflexion and spin diffusion.Comment: 9 pages, 9 figures, RevTe

We have measured local and non-local conductance of mesoscopic normal-metal/superconductor hybrid structures fabricated by e-beam lithography and shadow evaporation. The sample geometry consists of a superconducting aluminum bar with two normal-metal wires forming tunnel contacts to the aluminum at distances of the order of the superconducting coherence length. We observe subgap anomalies in both local and non-local conductance that quickly decay with magnetic field and temperature. For the non-local conductance both positive and negative signs are found as a function of bias conditions, indicating at a competition of crossed Andreev reflection and elastic cotunneling. Our data suggest that the signals are caused by a phase-coherent enhancement of transport rather than dynamical Coulomb blockade.