Single crystal neutron diffraction, inelastic neutron scattering and electron spin resonance experiments are used to study the magnetic structure and spin waves in Pb2VO(PO4)2, a prototypical layered S = 1/2 ferromagnet with frustrating next nearest neighbor antiferromagnetic interactions. The observed excitation spectrum is found to be inconsistent with a simple square lattice model previously proposed for this material. At least four distinct exchange coupling constants are required to reproduce the measured spin wave dispersion. The degree of magnetic frustration is correspondingly revised and found to be substantially smaller than in all previous estimates.arXiv :1902.11172v2 [cond-mat.str-el]
Magnetization, magnetic torque, neutron diffraction and NMR experiments are used to map out the H−T phase diagram of the prototypical quasi-two-dimensional ferro-antiferromagnet Pb2VO(PO4)2 in magnetic fields up to 27 T. When the field is applied perpendicular to the axis of magnetic anisotropy, a new magnetic state emerges through a discontinuous transition and persists in a narrow field range just below saturation. The measured NMR spectra suggest a complex and possibly incommensurate magnetic order in that regime.
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