We report a novel method to unambiguously determine the magnitude and orientation of linear dichroism in a simultaneous way. It is based on the use of a dedicated dual-frequency dual-polarization coherent source providing two orthogonal circularly polarized modes at the output. We show that the interaction of such a beam with dichroic media gives rise to a beatnote signal whose amplitude and phase enable the full determination of the diattenuation coefficient and axis orientation, respectively. The application of this method to polarimetric imaging provides single-shot sample characterization by its diattenuation coefficient and optical axis angle, with potential applications in biomedical imaging.

Polarimetric sensing by orthogonality breaking has been recently proposed as an alternative technique for performing direct and fast polarimetric measurements using a specific dual-frequency dual-polarization (DFDP) source. Based on the instantaneous Stokes-Mueller formalism to describe the high-frequency evolution of the DFDP beam intensity, we thoroughly analyze the interaction of such a beam with birefringent, dichroic and depolarizing samples. This allows us to confirm that orthogonality breaking is produced by the sample diattenuation, whereas this technique is immune to both birefringence and diagonal depolarization. We further analyze the robustness of this technique when polarimetric sensing is performed through a birefringent waveguide, and the optimal DFDP source configuration for fiber-based endoscopic measurements is subsequently identified. Finally, we consider a stochastic depolarization model based on an ensemble of random linear diattenuators, which makes it possible to understand the progressive vanishing of the detected orthogonality breaking signal as the spatial heterogeneity of the sample increases, thus confirming the insensitivity of this method to diagonal depolarization. The fact that the orthogonality breaking signal is exclusively due to the sample dichroism is an advantageous feature for the precise decoupled characterization of such an anisotropic parameter in samples showing several simultaneous effects.

We report the design and optimization of an active polarimetric imaging demonstrator operating at 1.55 μm that is based on the orthogonality breaking technique. It relies on the use of a fibered dual-frequency dual-polarization source raster scanned over the scene. A dedicated opto-electronic detection chain is developed to demodulate the optical signal backscattered at each location of the scene in real time, providing multivariate polarimetric image data in one single scan with limited acquisition time. We experimentally show on a homemade scene that contrast maps can be built to reveal hidden dichroic objects over a depolarizing background, as well as their orientation. Finally, experiments through air turbulence illustrate the benefit of such an imaging architecture over standard polarimetric techniques requiring multiple image acquisitions.