Colloidal quantum dots (QDs) are an attractive light source for visible photonics, in particular their widely tunable emission wavelength, inexpensive wet-chemical synthesis and straight-forward hybrid integration can make the difference. In this work, integrated light-emitting diodes are demonstrated based on CdSe/CdS QDs, with the emission directly coupled to a silicon nitride waveguide. The devices feature a record current density of up to 100 A cm −2 and a maximum on-chip power density of almost 1.5 W cm −2 in a single-mode waveguide. Operated as detectors, the photodiodes have a low dark current of 1.5 µA cm −2 . It is anticipated, that the devices will find an application in chip-based absorption spectroscopy and bio-sensing, as they can be post-processed on foundry-fabricated waveguide platforms, at a low cost. In addition, this approach provides the missing low-loss waveguide layer, necessary for building an electrically pumped laser using colloidal QDs.
Colloidal quantum dots (QDs) have become an attractive light source for visible photonics. Here, we demonstrate the first integrated LED based on CdSe/CdS QDs, with the emission directly coupled to a silicon nitride waveguide.
Colloidal quantum dots (QDs) are excellent optical gain materials that combine high material gain, a strong absorption of pump light, stability under strong light exposure and a suitability for solution-based processing. The integration of QDs in laser cavities that fully exploit the potential of these emerging optical materials remains, however, a challenge. In this work, we report on a vertical cavity surface emitting laser, which consists of a thin film of QDs embedded between two layers of polymerized chiral liquid crystal. Forward directed, circularly polarized defect mode lasing under nanosecond-pulsed excitation is demonstrated within the photonic band gap of the chiral liquid crystal. Stable and long-term narrow-linewidth lasing of an exfoliated free-standing, flexible film under water is obtained at room temperature. Moreover, we show that the lasing wavelength of this flexible cavity shifts under influence of pressure, strain or temperature. As such, the combination of solution processable and stable inorganic QDs with high chiral liquid crystal reflectivity and effective polymer encapsulation leads to a flexible device with long operational lifetime, that can be immersed in different protic solvents to act as a sensor.
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