The root-mean-square (rms) nuclear charge radius of 8 He, the most neutron-rich of all particlestable nuclei, has been determined for the first time to be 1.93(3) fm. In addition, the rms charge radius of 6 He was measured to be 2.068(11) fm, in excellent agreement with a previous result.The significant reduction in charge radius from 6 He to 8 He is an indication of the change in the correlations of the excess neutrons and is consistent with the 8 He neutron halo structure. The experiment was based on laser spectroscopy of individual helium atoms cooled and confined in a magneto-optical trap. Charge radii were extracted from the measured isotope shifts with the help of precision atomic theory calculations. * Electronic address: pmueller@anl.gov 1

a b s t r a c tProof-of-principle of a new mass spectrometric technique for radiocarbon measurement is demonstrated. Interfering nitrogen and hydrocarbon molecules are largely eliminated in a charge-exchange cell operating on non-metallic gas. The positive-to-negative ion conversion is the reverse of that conventionally used in accelerator mass spectrometry (AMS) and is compatible with plasma ion sources that may be significantly more efficient and capable of greater output than are AMS sputter ion sources. The Nanogan electron cyclotron resonance (ECR) ion source employed exhibited no sample memory and the >50 kyrs age range of AMS was reproduced. A bespoke prototype new instrument is now required to optimise the plasma and cell physics and to realise hypothetical performance gains over AMS.

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