We studied the phenomenon of relatively small changes in the energy of ultracold neutrons (UCN) (when compared to thermal motion energy) when these are reflected on a surface. The changes observed involved both increases in UCN energy (their heating) and decreases (cooling) of the order of ~ 10-7 eV. The probability values of this process on various surfaces ranged between 10-8 and 10-5 per one collision; the probability of such a small heating was many times larger than that of such a small cooling. We measured the spectra of such heated neutrons and the dependence of small heating probability on the temperature of sample out-gazing. We found that out-gazing of samples in vacuum at a temperature of 500–600 K could increase the small heating probability on stainless steel surface by a factor of ~ 100; and on copper surface by a factor of ~ 10. We observed, for the first time, extremely intensive small heating of UCN on powder of diamond nanoparticles. Neither small heating of UCN, nor nanoparticles could be found on a sapphire single crystal surface. This set of experimental data indicates that the inelastic scattering of UCN on weakly bound nanoparticles at a surface in a state of thermal motion is responsible for the process investigated.

No abstract

If the wavelength of radiation and the size of inhomogeneities in the medium are approximately equal, the radiation might be intensively scattered in the medium and reflected from its surface. Such efficient nanomaterial reflectors are of great scientific and technological interest. In previous works, we demonstrated a significant improvement in the efficiency of reflection of slow neutrons from a powder of diamond nanoparticles by replacing hydrogen located on the surface of nanoparticles with fluorine and removing the residual sp2 amorphous shells of nanoparticles via the fluorination process. In this paper, we study the mechanism of this improvement using a set of complementary experimental techniques. To analyze the data on a small-angle scattering of neutrons and X-rays in powders of diamond nanoparticles, we have developed a model of discrete-size diamond nanospheres. Our results show that fluorination does not destroy either the crystalline cores of nanoparticles or their clustering in the scale range of 0.6–200 nm. This observation implies that it does not significantly affect the neutron scattering properties of the powder. We conclude that the overall increase in reflectivity from the fluorinated nanodiamond powder is primarily due to the large reduction of neutron losses in the powder caused by the removal of hydrogen contaminations.

Diamond, with its exceptionally high optical nuclear potential and low absorption cross-section, is a unique material for a series of applications in VCN (very cold neutron) physics and techniques. In particular, powder of diamond nanoparticles provides the best reflector for neutrons in the complete VCN energy range. It allowed also the first observation of quasi-specular reflection of cold neutrons (CN) from disordered medium. Effective critical velocity for such a quasi-specular reflection is higher than that for the best super-mirror. Nano-diamonds survive in high radiation fluxes; therefore they could be used, under certain conditions, in the vicinity of intense neutron sources.

We propose to perform the first measurement of the neutron–neutron scattering cross section in the through-channel of the pulsed aperiodic reactor YAGUAR (Snezhinsk, Russia). Such a measurement directly determines the neutron–neutron scattering length, and by comparison with the proton–proton scattering length bears upon the issue of charge symmetry of the nuclear force. The proposed experimental set-up, as well as modelling of the neutron density and of the frequency of neutron–neutron collisions is described. Experimental results are reported on the formation and optimization of the thermal neutron field inside the through-channel of the reactor YAGUAR. The instantaneous value of 1.1 × 1018 cm−2 s−1 obtained for the thermal neutron flux density is large enough to perform the first direct neutron–neutron scattering length measurement.