Annual dose on the containment building wall of the interim storage facility at normal condition was calculated to estimate the dose rate transition of the facility of PWR spent nuclear fuel. In this study, source term was generated by ORIGEN-ARP with 4.5 wt% initial enrichment, 45,000 MWd/MTU burnup and 10 years cooling time. Modeling of the storage facility and the containment building and radiation shielding evaluations were conducted by MCNP code depending on the distance between the wall and the facility in the building. In the case of the centralized storage system, the distance required for the annual dose rate limit from 10CFR72 was estimated to be 50 m.

Background: Aptamers are currently being used in various fields including medical treatments due to their characteristics of selectively binding to specific molecules. Due to their special characteristics, the aptamers are expected to be used to remove radionuclides from a large amount of liquid radioactive waste generated during the decommissioning of nuclear power plants. The radiological effects on the aptamers should be evaluated to ensure their integrity for the application of a radionuclide removal technique.Materials and Methods: In this study, Monte Carlo N-Particle transport code version 6 (MCNP6) and Monte Carlo damage simulation (MCDS) codes were employed to evaluate the radiological effects on the aptamers. MCNP6 was used to evaluate the secondary electron spectrum and the absorbed dose in a medium. MCDS was used to calculate the DNA damage by using the secondary electron spectrum and the absorbed dose. Binding experiments were conducted to indirectly verify the results derived by MCNP6 and MCDS calculations.Results and Discussion: Damage yields of about 5.00×10^-4 were calculated for 100 bp aptamer due to the radiation dose of 1 Gy. In experiments with radioactive materials, the results that the removal rate of the radioactive ⁶⁰Co by the aptamer is the same with the non-radioactive ⁵⁹Co prove the accuracy of the previous DNA damage calculation.Conclusion: The evaluation results suggest that only very small fraction of significant number of the aptamers will be damaged by the radioactive materials in the liquid radioactive waste. Keywords: Aptamer, Liquid Radioactive Waste, Decommissioning, Decontamination, Radiological Damage

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