Atmospheric-pressure plasmas (APPs) have attracted great interest and have been widely applied in biomedical applications, as due to their non-thermal and reactive properties, they interact with living tissues, cells and bacteria. Various types of plasma sources generated at atmospheric pressure have been developed to achieve better performance in specific applications. This article presents an overview of the general characteristics of APPs and a brief summary of their biomedical applications, and reviews a wide range of these sources developed for biomedical applications. The plasma sources are classified according to their power sources and cover a wide frequency spectrum from dc to microwaves. The configurations and characteristics of plasma sources are outlined and their biomedical applications are presented.
As interest has increased in the interaction between low-temperature plasmas and living cells or organic materials, the role of modelling and simulation of atmospheric pressure plasmas has become important in understanding the effects of charged particles and radicals in biomedical applications. This review paper introduces the general properties of low-temperature atmospheric pressure plasma devices for biomedical applications and explains recently reported simulation results. Control parameters of atmospheric pressure plasmas, such as gas mixture composition, driving frequency and voltage and the function shape of sinusoidal and pulsed power, are considered through both a review of previous findings and new simulation results in order to improve plasma properties for given purposes. Furthermore, the simulation or modelling techniques are explained along with surface interactions of the plasma for the future development of simulation codes to study the interaction of plasmas with living cells.
Abstract2D tin‐based perovskites have gained considerable attention for use in diverse optoelectronic applications, such as solar cells, lasers, and thin‐film transistors (TFTs), owing to their good stability and optoelectronic properties. However, their intrinsic charge‐transport properties are limited, and the insulating bulky organic ligands hinder the achievement of high‐mobility electronics. Blending 3D counterparts into 2D perovskites to form 2D/3D hybrid structures is a synergistic approach that combine the high mobility and stability of 3D and 2D perovskites, respectively. In this study, reliable p‐channel 2D/3D tin‐based hybrid perovskite TFTs comprising 3D formamidinium tin iodide (FASnI3) and 2D fluorinated 4‐fluoro‐phenethylammonium tin iodide ((4‐FPEA)2SnI4) are reported. The optimized FPEA‐incorporated TFTs show a high hole mobility of 12 cm2 V−1 s−1, an on/off current ratio of over 108, and a subthreshold swing of 0.09 V dec−1 with negligible hysteresis. This excellent p‐type characteristic is compatible with n‐type metal‐oxide TFT for constructing complementary electronics. Two procedures of antisolvent engineering and device patterning are further proposed to address the key concern of low‐performance reproducibility of perovskite TFTs. This study provides an alternative A‐cation engineering method for achieving high‐performance and reliable tin‐halide perovskite electronics.
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