We report on the efficient design of quantum optimal control protocols to manipulate the motional states of an atomic Bose-Einstein condensate (BEC) in a one-dimensional optical lattice. Our protocols operate on the momentum comb associated with the lattice. In contrast to previous works also dealing with control in discrete and large Hilbert spaces, our control schemes allow us to reach a wide variety of targets by varying a single parameter, the lattice position. With this technique, we experimentally demonstrate a precise, robust and versatile control: we optimize the transfer of the BEC to a single or multiple quantized momentum states with full control on the relative phase between the different momentum components. This also allows us to prepare the BEC in a given eigenstate of the lattice band structure, or superposition thereof.

The field of quantum simulation, which aims at using a tunable quantum system to simulate another, has been developing fast in the past years as an alternative to the all-purpose quantum computer. So far, most efforts in this domain have been directed to either fully regular or fully chaotic systems. Here, we focus on the intermediate regime, where regular orbits are surrounded by a large sea of chaotic trajectories. We observe a quantum chaos transport mechanism, called chaos-assisted tunneling, that translates in sharp resonances of the tunneling rate and provides previously unexplored possibilities for quantum simulation. More specifically, using Bose-Einstein condensates in a driven optical lattice, we experimentally demonstrate and characterize these resonances. Our work paves the way for quantum simulations with long-range transport and quantum control through complexity.