Pressure sensors urgently need high-performance sensing materials in order to be developed further. Sensitivity and creep are regarded as two key indices for assessing a sensor’s performance. For the design and optimization of sensing materials, an accurate estimation of the impact of several parameters on sensitivity and creep is essential. In this study, sensitivity and creep were predicted using the response surface methodology (RSM) and support vector regression (SVR), respectively. The input parameters were the concentrations of nickel (Ni) particles, multiwalled carbon nanotubes (MWCNTs), and multilayer graphene (MLG), as well as the magnetic field intensity (B). According to statistical measures, the SVR model exhibited a greater level of predictability and accuracy. The non-dominated sorting genetic-II algorithm (NSGA-II) was used to generate the Pareto-optimal fronts, and decision-making was used to determine the final optimal solution. With these conditions, the optimized results revealed an improved performance compared to the earlier study, with an average sensitivity of 0.059 kPa−1 in the pressure range of 0–16 kPa and a creep of 0.0325, which showed better sensitivity in a wider range compared to previous work. The theoretical sensitivity and creep were relatively similar to the actual values, with relative deviations of 0.317% and 0.307% after simulation and experimental verification. Future research for transducer performance optimization can make use of the provided methodology because it is representative.

Response surface methodology (RSM) and central composite design (CCD) were used to improve the preparation of carbon nanotube and graphene (CNT-GN)-sensing unit composite materials in this study. Four independent variable factors (CNT content, GN content, mixing time, and curing temperature) were controlled at five levels, and 30 samples were generated using the multivariate control analysis technique. On the basis of the experimental design, semi-empirical equations were developed and utilized to predict the sensitivity and compression modulus of the generated samples. The results reveal a strong correlation between the experimental and expected values of sensitivity and the compression modulus for the CNT-GN/RTV (room-temperature-vulcanized silicone rubber) polymer nanocomposites fabricated using different design strategies. The correlation coefficients for the sensitivity and compression modulus are R2 =0.9634 and R2=0.9115, respectively. The ideal preparation parameters of the composite in the experimental range include a CNT content of 1.1 g, a GN content of 1.0 g, a mixing time of 15 min, and a curing temperature of 68.6 °C, according to theoretical predictions and experimental findings. At 0~30 kPa, the CNT-GN/RTV-sensing unit composite materials may reach a sensitivity of 0.385 kPa−1 and a compressive modulus of 601.567 kPa. This provides a new idea for the preparation of flexible sensor cells and reduces the time and economic cost of experiments.

Polymer creep can significantly reduce the safety and dependability of composite applications, restricting their development and use in additional fields. In this study, single-factor and multi-factor analysis techniques were employed to systematically explore the impacts of nickel powder and graphene on the resistive creep of sensing units. The creep model between the rate of resistance changes and the pressure was established, and the material ratio was optimized to obtain a high creep resistance. The results demonstrated that the creep resistance was best when the filling particle was 10 wt.% and the ratio of nickel powder to graphene was 4:21, which was approximately 60% and 45% lower than the filling alone and the composite filling before optimization, respectively; the R2 of the theoretical value of the resistance creep model and the experimental value of the creep before and after optimization was 0.9736 and 0.9812, indicating that the resistance creep model was highly accurate. Consequently, the addition of filler particles with acceptable proportions, varied shapes, and different characteristics to polymers can effectively reduce polymer creep and has significant potential for the manufacture of sensing units for tactile sensors.