The fusion of 6 He with a 209 Bi target has been studied at energies near to and below the Coulomb barrier. Despite the weak binding of the valence neutrons in 6 He, little evidence is found for suppression of fusion due to projectile breakup. Instead, a large enhancement of sub-barrier fusion is observed. It is suggested that this enhancement may arise from coupling to positive Q value neutron transfer channels, resulting in "neutron flow" between the projectile and the target. [S0031-9007 (98)07674-1] PACS numbers: 25.60.Pj, 25.70.JjRecent theoretical studies of near-barrier and subbarrier fusion of the exotic "neutron halo" system 11 Li with 208 Pb (see, e.g., [1][2][3][4][5]) have generated a considerable amount of interest and controversy. The 11 Li nucleus contains two valence neutrons that are only very weakly coupled to a relatively tightly bound 9 Li core. This unusual composition manifests itself in both the structure of the nucleus, as in the existence of the neutron halo and of low-lying E1 modes [6], and also in reactions with other nuclei. Furthermore, neither the n-9 Li nor the n-n subsystems of 11 Li are bound, so that particle stability in this nucleus is achieved via three-body interactions. Systems of this kind, referred to as "Borromean" nuclei [7], provide an unusual opportunity to study three-body interactions in the nucleus.It has been known for some time that sub-barrier fusion of stable nuclei can be enhanced by several orders of magnitude beyond expectations from simple one-dimensional barrier penetration calculations. A qualitative understanding of this phenomenon has been achieved in terms of couplings to internal degrees of freedom of the target and projectile [8], resulting in a lowering of the effective fusion barrier. This dynamical effect is a very sensitive probe of the nuclear structure of the colliding partners. A lowering of the barrier, by 20% or more, is also a general feature in the results for 11 Li 1 208 Pb fusion presented in [1][2][3][4][5], but the leading effect that was calculated in this case is a static one, resulting from the larger radius of the 11 Li "halo" wave function which allows the attractive nuclear force to act at longer distances. However, additional dynamical enhancement was obtained from the coupling to the soft E1 mode [1,2]. The role played by projectile breakup channels, which are possibly important due to the weak binding of the valence neutrons, is considerably more controversial. Several groups [2][3][4] have reported that coupling to these channels reduces the fusion cross section near the barrier, leading to intriguing structure in the excitation function in this region. However, this point of view has been criticized by Dasso and Vitturi [5] who suggest that it results from a misunderstanding of the nature of multidimensional quantum-mechanical tunneling processes. They report only enhancement of the fusion yield, even in the presence of strong breakup channels. It is important to resolve this controversy since the competition between project...

Per- and polyfluoroalkyl substances (PFASs) are highly persistent synthetic chemicals, some of which have been associated with cancer, developmental toxicity, immunotoxicity, and other health effects. PFASs in grease-resistant food packaging can leach into food and increase dietary exposure. We collected ~400 samples of food contact papers, paperboard containers, and beverage containers from fast food restaurants throughout the United States and measured total fluorine using particle-induced γ-ray emission (PIGE) spectroscopy. PIGE can rapidly and inexpensively measure total fluorine in solid-phase samples. We found that 46% of food contact papers and 20% of paperboard samples contained detectable fluorine (>16 nmol/cm2). Liquid chromatography/high-resolution mass spectrometry analysis of a subset of 20 samples found perfluorocarboxylates, perfluorosulfonates, and other known PFASs and/or unidentified polyfluorinated compounds (based on nontargeted analysis). The total peak area for PFASs was higher in 70% of samples (10 of 14) with a total fluorine level of >200 nmol/cm2 compared to six samples with a total fluorine level of <16 nmol/cm2. Samples with high total fluorine levels but low levels of measured PFASs may contain volatile PFASs, PFAS polymers, newer replacement PFASs, or other fluorinated compounds. The prevalence of fluorinated chemicals in fast food packaging demonstrates their potentially significant contribution to dietary PFAS exposure and environmental contamination during production and disposal.

Multi-fragment decays of 129 Xe, 197 Au, and 238 U projectiles in collisions with Be, C, Al, Cu, In, Au, and U targets at energies between E/A = 400 MeV and 1000 MeV have been studied with the ALADIN forward-spectrometer at SIS. By adding an array of 84 SiCsI(Tl) telescopes the solid-angle coverage of the setup was extended to θ lab = 16 • . This permitted the complete detection of fragments from the projectile-spectator source.The dominant feature of the systematic set of data is the Z bound universality that is obeyed by the fragment multiplicities and correlations. These observables are invariant with respect to the entrance channel if plotted as a function of Z bound , where Z bound is the sum of the atomic numbers Z i of all projectile fragments with Z i ≥ 2. No significant dependence on the bombarding energy nor on the target mass is observed. The dependence of the fragment multiplicity on the projectile mass follows a linear scaling law.The reasons for and the limits of the observed universality of spectator fragmentation are explored within the realm of the available data and with model studies. It is found that the universal properties should persist up to much higher bombarding energies than explored in this work and that they are consistent with universal features exhibited by the intranuclear cascade and statistical multifragmentation models.

The growth of accelerator mass spectrometry as a tool for quantitative isotope ratio analysis in the biosciences necessitates high-throughput sample preparation. A method has been developed to convert CO(2) obtained from carbonaceous samples to solid graphite for highly sensitive and precise (14)C quantification. Septa-sealed vials are used along with commercially available disposable materials, eliminating sample cross contamination, minimizing complex handling, and keeping per sample costs low. Samples containing between 0.25 and 10 mg of total carbon can be reduced to graphite in approximately 4 h in routine operation. Approximately 150 samples per 8-h day can be prepared by a single technician.

The neutron unbound ground state of (25)O (Z=8, N=17) was observed for the first time in a proton knockout reaction from a (26)F beam. A single resonance was found in the invariant mass spectrum corresponding to a neutron decay energy of 770_+20(-10) keV with a total width of 172(30) keV. The N=16 shell gap was established to be 4.86(13) MeV by the energy difference between the nu1s(1/2) and nu0d(3/2) orbitals. The neutron separation energies for (25)O agree with the calculations of the universal sd shell model interaction. This interaction incorrectly predicts an (26)O ground state that is bound to two-neutron decay by 1 MeV, leading to a discrepancy between the theoretical calculations and experiment as to the particle stability of (26)O. The observed decay width was found to be on the order of a factor of 2 larger than the calculated single-particle width using a Woods-Saxon potential.