The partially coherent Lorentz-Gauss vortex beam generated by a Schell-model source has been introduced. Based on the extended Huygens-Fresnel principle, the cross-spectral density function of a partially coherent Lorentz-Gauss vortex beam propagating in oceanic turbulence is derived. The influences of coherence length, topological charge M, and oceanic turbulence on the spreading properties and position of the coherence vortex for a partially coherent Lorentz-Gauss vortex beam are analyzed in detail. The results show that a partially coherent Lorentz-Gauss vortex beam propagating in stronger oceanic turbulence will evolve into a Gaussian-like beam more rapidly as the propagation distance increases, and the number of coherent vortices will change.
Based on the extended Huygens-Fresnel principle, the analytical expressions for partially coherent fourpetal Gaussian vortex beams propagating in oceanic turbulence are obtained, and the influence of the coherence length, beam order N, topological charge M and oceanic turbulence parameters on the evolution properties of beams are discussed in detail using numerical examples. The results show that the beam will evolve into a Gausslike beam rapidly with decreasing coherence length σ and oceanic parameters ς and ε, or increasing oceanic parameter T χ in the far field due to the influence of the coherence length and oceanic turbulence.
The effects of different bridging fluorene units on the two-photon absorption (TPA) properties and ultrafast response of organic conjugated oligomers were investigated for three star-shaped oligomers named TFT-1, TFT-2 and TFT-3. These three oligomers are composed of the same central core 1,3,5-triazine, with three arms that consist of specific numbers of bridging fluorene groups and with triphenylamine as electrondonating group at the terminal end of each arm. The studies on these oligomers were carried out by using two-photon excited fluorescence (TPF), degenerate pump-probe techniques, transient absorption spectroscopy and time-resolved photoluminescence (TRPL) methods. The TPA cross-sections were determined to be 1509 GM, 1260 GM and 789 GM for TFT-1, TFT-2 and TFT-3, respectively, decreasing with the increase of bridging fluorene number. Ultrafast dynamics results show that there is a fast intramolecular charge transfer (ICT) formation time of about several ps and a relatively long decay process of the ICT state. The formation time of ICT was found to increase from TFT-1 (1.9 ps), to TFT-2 (3.0 ps) and TFT-3 (6.3 ps), with the increased number of the fluorene bridge, which may explain the action of fluorene bridge on the electron transmission properties, the ICT properties and the TPA behavior.
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