STIRAP (Stimulated Raman Adiabatic Passage) is a powerful laser-based method, usually involving two photons, for efficient and selective transfer of population between quantum states. A particularly interesting feature is the fact that the coupling between the initial and the final quantum states is via an intermediate state even though the lifetime of the latter can be much shorter than the interaction time with the laser radiation. Nevertheless, spontaneous emission from the intermediate state is prevented by quantum interference. Maintaining the coherence between the initial and final state throughout the transfer process is crucial.STIRAP was initially developed with applications in chemical dynamics in mind. That is why the original paper of 1990 was published in The Journal of Chemical Physics. However, as of about the year 2000, the unique capabilities of STIRAP and its robustness with respect to small variations of some experimental parameters stimulated many researchers to apply the scheme in a variety of other fields of physics. The successes of these efforts are documented in this collection of articles. In Part A the experimental success of STIRAP in manipulating or controlling molecules, photons, ions or even quantum systems in a solid-state environment is documented. After a brief introduction to the basic physics of STIRAP, the central role of the method in the formation of ultra-cold molecules is discussed, followed by a presentation of how precision experiments (measurement of the upper limit of the electric dipole moment of the electron or detecting the consequences of parity violation in chiral molecules) or chemical dynamics studies at ultra-low temperatures benefit from STIRAP. Next comes the STIRAP-based control of photons in cavities followed by a group of three contributions which highlight the potential of the STIRAP concept in classical physics by presenting data on the transfer of waves (photonic, magnonic and phononic) between respective wave guides. The works on ions or ion-strings discuss options for applications e.g. in quantum information. Finally, the success of STIRAP in the controlled manipulation of quantum states in solid-state systems, which are usually hostile towards coherent processes, is presented, dealing with data storage in rare-earth ion doped crystals and in NV-centers or even in superconducting quantum circuits. The works on ions and those involving solid-state systems emphasize the relevance of the results for quantum information protocols.Part B deals with theoretical work including further concepts relevant for quantum information or invoking STIRAP for the manipulation of matter waves. The subsequent articles discuss experiments underway to demonstrate the potential of STIRAP for populating otherwise inaccessible high-lying Rydberg states of molecules, or controlling and cooling the translational motion of particles in a molecular beam or the polarization of angular momentum states. The series of articles concludes with a more speculative application of STIRAP i...
The reflection (or ‘mirror’) symmetry of space is among the fundamental symmetries of physics. It is connected to the conservation law for the quantum number purity and its violation and has a fundamental relation to stereochemistry and molecular chirality.
We present a novel architecture for a multi-pass amplifier based on a succession of optical Fourier transforms and short propagations that shows a superior stability for variations of the thermal lens compared to state-of-the-art 4fbased amplifiers. We found that the proposed multi-pass amplifier is robust to variations of the active medium dioptric power. The superiority of the proposed architecture is demonstrated by analyzing the variations of the size and divergence of the output beam in form of a Taylor expansion around the design value for variations of the thermal lens in the active medium. The dependence of the output beam divergence and size is investigated also for variations of the number of passes, for aperture effects in the active medium and as a function of the size of the beam on the active medium. This architecture makes efficient use of the transverse beam filtering inherent in the active medium to deliver a beam with excellent quality (TEM00).
We present the current status for the direct measurement of the positronium hyperfine structure using the 2 3 S1 → 2 1 S0 transition. This experiment, currently being commissioned at the slow positron beam facility at ETH Zurich, will be the first measurement of this transition and the first positronium hyperfine splitting experiment conducted in vacuum altogether. This experiment will be free of systematic effects found in earlier experiments, namely the inhomogeneity in static magnetic fields and the extrapolation from dense gases to vacuum. The achievable precision is expected to be on the order of 10 ppm while the systematic uncertainty is estimated to be within a few ppm. This would allow to check recent bound state QED calculations and a 3σ discrepancy with earlier experiments.1 Such corrections enter in higher order loop processes, but this is strongly suppressed. arXiv:1805.05886v3 [physics.atom-ph]
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