X-ray diffraction was used to study the formation and structure of mixed ferrite Li 0X5À0X5x Cu x ± Fe 2X5À0X5x O 4 (where x 0, 0.1, 0.3, 0.5, 0.7, 0.9 and 1.0). The X-ray diffraction pattern proved that the prepared samples were formed in the spinel structure. The samples with x 0X7 have cubic structure while the samples with x 0X9, 1 have tetragonal structure. The experimental and theoretical lattice parameters a exp and a th ) were calculated for each composition. A comparison study between experimental and theoretical values was performed. The initial permeability m i was measured as a function of temperature for the above-investigated ferrite. Utilizing the initial permeability data, the Curie temperature T C was determined. T C was found to decrease with increasing Cu 2 ion content. The anomaly seen in the temperature dependence of m i was attributed to the existence of two structural phases (cubic and tetragonal phase). The magnetization M was measured at room temperature in the range of magnetizing field from 0 to 1307 Am À1 . The calculated relative permeability showed a dependence on the magnetizing field and composition. In addition, the B H loop was measured at room temperature and at constant magnetizing field H 350 Am À1 . The coercive force H c , remanence induction B r and the apparent loss energy P s were estimated. It has been found that both B r and P s are composition dependent while H c is independent of composition.