We have measured the magnetotransmission of thin film samples of YBa 2 Cu 3 O 7 in the normal state using circularly polarized light at frequencies from 15 to 180 cm 21 . The magneto-optical signal is consistent with the ac Hall effect of holes with a reduced scattering rate and an enhanced mass compared to the zero-field transport parameters. This result agrees with a simple high-frequency extension of models which have been developed to explain the anomalous dc Hall effect in the normal state of high-T c superconductors. PACS numbers: 78.20.Ls, 72.15.Gd, 74.72.Bk The nature of the ab-plane charge carrier dynamics in the normal state of YBa 2 Cu 3 O 7 is currently as intriguing a subject as the mechanism responsible for the superconductivity below T c . Hall measurements have revealed the charge carriers to be holes with a density related to the oxygen doping level, but there the resemblance to simple metals ends. A striking T 2 behavior of the inverse Hall angle cot u H s xx ͞s xy has been observed in many different types of samples [1][2][3][4]. In addition, the ac conductivity, derived from broadband optical reflectivity measurements [5,6], shows distinctly non-Drude-like behavior above 200 cm 21 . On the other hand, previous far-infrared (FIR) magnetotransmission measurements of YBa 2 Cu 3 O 7 in the superconducting state [7] have found a signal consistent with cyclotron resonance of free holes with a mass m c of ͑3.1 6 0.5͒m e .In this Letter we measure the FIR magneto-optical activity of YBa 2 Cu 3 O 7 thin films at 9 T and 95 K, where v c t ϳ 1͞40, so that we observe an overdamped cyclotron resonance response, or more appropriately the ac Hall effect. The signal is consistent with a holelike Hall effect, but fitting the data with a Drude model requires a smaller scattering rate and larger mass then the zero-field values. This result is understood by extending the ideas of Anderson [1,2] or Carrington et al. [3,4], used to explain the temperature dependence of the dc Hall effect, to high frequencies. In these theories, the Hall effect is dependent upon a scattering time and mass which are distinct from the ordinary transport quantities and are associated with spinons, or carriers near the corners of the 2D Fermi surface, respectively. Other phenomenological theories have also been proposed to explain the appearance of two scattering times in the charge dynamics of cuprate materials [8].Two types of thin film samples were used in these studies. High quality films of YBa 2 Cu 3 O 7 were produced by precursor deposition onto (100) LaAlO 3 substrates, followed by postannealing at 800 ± C in a wet oxygen atmosphere. Such films have proven to be of higher quality than typical laser-deposited samples, in terms of their degree of crystallinity and low defect density [9]. The superconducting transitions were characterized by dc resistivity and ac susceptibility measurements and found to be typically 92 6 0.3 K. Another class of samples were grown by pulsed laser deposition and in situ annealing on Si substrates ...
Far-infrared magnetotransmission measurements of normal-state thin films are discussed. The magneto-optical signals observed in circularly polarized light are consistent with the ac Hall effect of holes with a reduced scattering rate and an enhanced mass compared to the zero-field transport parameters. The results agree with a simple high-frequency extension of models which have been developed to explain the anomalous dc Hall effect in the normal state of high- superconductors in terms of two scattering rates. The Hall scattering rate , where and K. These experiments provide new tests of the Fermi-liquid versus non-Fermi-liquid nature of these materials.
The magneto-optical activity of superconducting YBa2Cu3O7 observed by Karrai et al. is not present in many commonly employed models of vortex dynamics. Here we propose a simple, unifying picture for the frequency dependent magneto-optic response of type-II superconductors at low temperatures. We bring together Kohn's theorem, vortex core excitations, and vortex pinning and damping into a single expression for the conductivity tensor. The theory describes magneto-optical activity observed in infrared transmission measurements of thin films of YBa2Cu3O7.PACS numbers: 74.25. Nf, 74.60.Ge, 74.25.Gz, 76.40.+b For applications of superconductivity vortex motion and pinning is of great importance. Many models for vortex dynamics have been developed such as those of Bardeen and Stephen [1], Nozieres and Vinen [2], and Clem and Coffey [3]. One way of studying vortex dynamics is to go to frequencies that are large compared with the characteristic frequencies associated with pinning and damping to observe the free inertial response of the vortices. This regime is not well studied and moreover a microscopic approach is needed. We note that, for high temperature superconductors, estimates [4] of the frequency range over which one expects electromagnetic absorption (10 10 − 10 14 s −1 ) overlaps with the microscopic energy scale associated with quantized quasiparticle states in vortex cores [5]. Because of the short coherence length in high temperature superconductors, the energy scale of quasi-particle states localized at the vortex core is large.These considerations have prompted a re-examination of vortex core states. Karrai et al. examined the magnetic field and frequency dependent infrared transmission coefficient of thin films of YBa 2 Cu 3 O 7 and found evidence for dipole transitions in vortex cores [6]. In addition, magneto-optical activity of the superconducting state was observed in these experiments [7]. For frequencies above the vortex resonance this chiral response is consistent with the cyclotron resonance of the mixed state. According to Kohn's theorem [8], for an isotropic, homogeneous electron system in a uniform applied magnetic field H, the only excitation produced by a uniform electrodynamic field is the cyclotron resonance at the frequency ω c = eH/mc, where m is the bare band mass.Thus, for an ideal, pure superconductor, cyclotron resonance is expected. From these considerations, one of the requirements of a theory of vortex dynamics is that it be consistent with Kohn's theorem. Commonly employed theories [1,3,4] fail this test since they are non-chiral.The matrix elements and selection rules for the dipole transitions in vortex cores have been studied by Jankó and Shore [9] and Zhu, Zhang and Drew [10]. Kopnin [11] proposed a peak in the electromagnetic absorption of pure superconductors due to these transitions. However Hsu [12,13] showed that these intravortex transitions are not excited by long wavelength probes in the clean limit. Instead the collective cyclotron motion of the center of mass i...
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