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Multifunctional sensing systems play important roles in a variety of applications, incluing health surveillance, intelligent prothetics, human–machine/ambinece interfaces, and many others. The richness of the signal and the decoupling among multiple parameters are essential for simultaneous, multimodal measurements. However, current multifunctional sensing fails to decouple interferences from various signals. Here, we propose a double-sided wearable system that both enables multifunctional sensing and avoids the interferences among multiple parameters. Specifically, the sensitivities of system modules to strain are controlled through customizing the pattern and morphology of sensing electrodes as well as the modification of active materials. Compensation of temperature drift and selection of sensing mechanisms ensure the thermal stability of the system. The encapsulation of modules resists the interferences of proximity, normal pressure, and gas molecules at the same time. A double-sided partition layout with serpentine interconnections reduces the effect of motion artifacts and ensures simultaneous operation of electrochemical-sensing modules. Cooperation among decoupled modules acts as the bridge between the perception of ambience changes and the timely feedback of the human body. In addition, to sense the signal at the interface, modules for energy harvesting and storage are also integrated into the system to broaden its application scenarios.

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