Meteorites contain relict decay products of short-lived radionuclides that were present in the protoplanetary disk when asteroids and planets formed. Several studies reported a high abundance of 60 Fe (t 1/2 =2.62±0.04 Myr) in chondrites ( 60 Fe/ 56 Fe~610 -7 ), suggesting that planetary materials incorporated fresh products of stellar nucleosynthesis ejected by one or several massive stars that exploded in the vicinity of the newborn Sun. We measured 58 Fe/ 54 Fe and 60 Ni/ 58 Ni isotope ratios in whole rocks and constituents of differentiated achondrites (ureilites, aubrites, HEDs, and angrites), unequilibrated ordinary chondrites Semarkona (LL3.0) and NWA 5717 (ungrouped petrologic type 3.05), metal-rich carbonaceous chondrite Gujba (CBa), and several other meteorites (CV, EL H, LL chondrites; IIIAB, IVA, IVB iron meteorites). We derive from these measurements a much lower initial 60 Fe/ 56 Fe ratio of (11.5±2.6)×10 -9 and conclude that 60 Fe was homogeneously distributed among planetary bodies. This low ratio is consistent with derivation of 60 Fe from galactic background ( 60 Fe/ 56 Fe≈2.810 -7 in the interstellar medium from -ray observations) and can be reconciled with high 26 Al/ 27 Al~5×10 -5 in chondrites if solar material was contaminated through winds by outer layers of one or several massive stars (e.g., a Wolf-Rayet star) rich in 26 Al and poor in 60 Fe. We present the first chronological application of the 60 Fe-60 Ni decay system to establish the time of core formation on Vesta at Myr after condensation of calcium-aluminum-rich inclusions (CAIs).
Carbonaceous meteorites are thought to be fragments of C-type (carbonaceous) asteroids. Samples of the C-type asteroid (162173) Ryugu were retrieved by the Hayabusa2 spacecraft. We measure the mineralogy, bulk chemical and isotopic compositions of Ryugu samples. They are mainly composed of materials similar to carbonaceous chondrite meteorites, particularly the CI (Ivuna-type) group. The samples consist predominantly of minerals formed in aqueous fluid on a parent planetesimal. The primary minerals were altered by fluids at a temperature of 37 ± 10°C, 5.2 − 0.8 + 0.7 (Stat.) − 2.1 + 1.6 (Syst.) million years after formation of the first solids in the Solar System. After aqueous alteration, the Ryugu samples were likely never heated above ~100°C. The samples have a chemical composition that more closely resembles the Sun’s photosphere than other natural samples do.
Silicon and Mg in differentiated rocky bodies exhibit heavy isotope enrichments that have been attributed to evaporation of partially or entirely molten planetesimals. We evaluate the mechanisms of planetesimal evaporation in the early solar system and the conditions that controled attendant isotope fractionations.Energy balance at the surface of a body accreted within ~1 Myr of CAI formation and heated from within by 26 Al decay results in internal temperatures exceeding the silicate solidus, producing a transient magma ocean with a thin surface boundary layer of order < 1 meter that would be subject to foundering. Bodies that are massive enough to form magma oceans by radioisotope decay (≥ 0.1% ) can retain hot rock vapor even in the absence of ambient nebular gas. We find that a steady-state rock vapor forms within minutes to hours and results from a balance between rates of magma evaporation and atmospheric escape. Vapor pressure buildup adjacent to the surfaces of the evaporating magmas would have inevitably led to an approach to equilibrium isotope partitioning between the vapor phase and the silicate melt. Numerical simulations of this near-equilibrium evaporation process for a body with a radius of ~ 700 km yield a steady-state far-field vapor pressure of 10 -8 bar and a vapor pressure at the surface of 10 -4 bar, corresponding to 95% saturation. Approaches to equilibrium isotope fractionation between vapor and melt should have been the norm during planet formation due to the formation of steady-state rock vapor atmospheres and/or the presence of protostellar gas.We model the Si and Mg isotopic composition of bulk Earth as a consequence of accretion of planetesimals that evaporated subject to the conditions described above. The results show that the best fit to bulk Earth is for a carbonaceous chondrite-like source material with about 12% loss of Mg and 15% loss of Si resulting from near-equilibrium evaporation into the solar protostellar disk of H 2 on timescales of 10 4 to 10 5 years. .
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