Highly efficient broadband absorbing surfaces covering the UV, visible and near-IR regions are of great importance for low-light imaging devices, optical devices and optoelectronic devices. In this work, we demonstrate the fabrication of remarkably efficient absorbing surfaces due to the formation of nanoflower-like cavity structures on a stainless steel (SS304) surface, along with micropatterning in a hierarchical fashion. The fabrication process is carried out using noncontact, programmable, single-step laser irradiation by an inexpensive and robust 532 nm nanosecond laser. The measured specular antireflection properties over a wide spectral region (250-1800 nm) are extremely low, less than 0.5%, over a large range of incident angles and for both orthogonal polarizations. These special hierarchical structures with nanorods, nanoparticles, and nanocavities, completely trap the photon incident on these surfaces due to multiple reflections. These surface structures evolve with time to give better nanostructured features with higher oxygen content on the surfaces, revealed by FESEM elemental analysis, which increases the ability to trap photons. We believe these antireflection surfaces, with high efficiencies and longterm stability, will play a vital role in many modern technological applications.
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