High sensitivity and a large quality factor (Q) are two desirable goals to achieve a high figure of merit (FoM) in refractive index (RI) sensing. However, simultaneously satisfying these two goals is challenging. Herein, we propose a new class of hybrid high-Q metasurfaces, which are dielectric arrays standing on a Au plasmonic nanofilm, possessing the advantages of both high RI sensitivity and a large Q. The hybrid metasurface can support the plasmon-coupled lattice mode, which has extremely narrow full width at half-maximum (fwhm) resulting in a high-Q. The hybrid metasurface can be fabricated by a facile straightforward lithography technique and exhibits ultrahigh FoM values over a wide RI range (1−1.384) due to its narrow fwhm (smaller than 1 nm) and tunable high RI sensitivity. The highest Q and FoM values of 2370 and 1431 were experimentally demonstrated, respectively, giving the proposed hybrid metasurface great potential for building advanced optical biosensors in future applications.
Employing nanostructure to generate large chiroptical response has been cultivated as an emerging field, for its great potentials in integrated optics, biochemistry detections, etc. However, the lack of intuitive approaches for analytically describing the chiroptical nanoparticles has discouraged researchers from effectively designing advanced chiroptical structures. In this work, we take the twisted nanorod dimer system as a basic example to provide an analytical approach from the perspective of mode coupling, including far-field coupling and near-field coupling of nanoparticles. Using this approach, we can calculate the expression of circular dichroism (CD) in the twisted nanorod dimer system, which can establish the analytical relationship between the chiroptical response and the basic parameters of this system. Our results show that the CD response can be engineered by modulating the structure parameters, and a high CD response of ∼ 0.78 under the guidance of this approach has been achieved.
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