No abstract

High-entropy alloy (HEA) superconductors—a new class of functional materials—can be utilized stably under extreme conditions, such as in space environments, owing to their high mechanical hardness and excellent irradiation tolerance. However, the feasibility of practical applications of HEA superconductors has not yet been demonstrated because the critical current density (Jc) for HEA superconductors has not yet been adequately characterized. Here, we report the fabrication of high-quality superconducting (SC) thin films of Ta–Nb–Hf–Zr–Ti HEAs via a pulsed laser deposition. The thin films exhibit a large Jc of >1 MA cm−2 at 4.2 K and are therefore favorable for SC devices as well as large-scale applications. In addition, they show extremely robust superconductivity to irradiation-induced disorder controlled by the dose of Kr-ion irradiation. The superconductivity of the HEA films is more than 1000 times more resistant to displacement damage than that of other promising superconductors with technological applications, such as MgB2, Nb3Sn, Fe-based superconductors, and high-Tc cuprate superconductors. These results demonstrate that HEA superconductors have considerable potential for use under extreme conditions, such as in aerospace applications, nuclear fusion reactors, and high-field SC magnets.

We investigate the effect of disorder on the superconducting mechanism of MgB2 thin films using low-energy ion irradiation. The c-axis lattice constant and T c of MgB2 thin films change systematically as the magnitude of disorder, which corresponds to the value of average displacements per atom (dpa avg), increases. Here, dpa avg is controlled by the amount of irradiated ions. The dpa avg dependence of the electron–phonon coupling constants (λ) is estimated using the McMillan equation. For dpa avg ⩽ 0.049, λ is linearly proportional to dpa avg. On the other hand, for dpa avg > 0.049, the T c of the disordered MgB2 deviates from the linear fitting curve, and insulating behavior is observed in the normal state resistivity. These results indicate that the superconducting mechanism of MgB2 can be changed by the electronic system caused by disorder strength affecting the electron–phonon coupling constant λ.

No abstract

High-entropy alloy (HEA) superconductors—a new class of functional materials—can be utilized stably under extreme conditions, such as in space environments, owing to their high mechanical hardness and excellent irradiation tolerance1–7. However, the feasibility of practical applications of HEA superconductors has not yet been demonstrated because the critical current density (Jc) for HEA superconductors has not yet been adequately characterized. Here, we report the fabrication of high-quality SC thin films of Ta–Nb–Hf–Zr–Ti HEAs via a pulsed laser deposition. The thin films exhibit a large Jc of > 1 MA cm−2 at 4.2 K and are therefore favorable for SC devices as well as large-scale applications. In addition, they show extremely robust superconductivity to irradiation-induced disorder controlled by the dose of Kr-ion irradiation. The superconductivity of the HEA films is more than 1000 times more resistant to displacement damage than that of other promising superconductors with technological applications, such as MgB2, Nb3Sn, Fe-based superconductors, and high-Tc cuprate superconductors. These results demonstrate that HEA superconductors have considerable potential for use under extreme conditions, such as in aerospace applications, nuclear fusion reactors, and high-field SC magnets.