The reservoir effect of Scandinavian sea water has been determined by dating seals and whales killed well before man's impact on the natural 14C concentration became significant. The samples were collected at different places along the Swedish coasts and in the Gulf of Finland. They derive from AD 1657 or 1658, 1868, 1875, 1894, and 1906. The EDTA treatment of bones was used to obtain collagen free from contaminants.An elk, originating from AD 1881 was selected for comparison. A seal from AD 1899 from the Caspian Sea was also included in the investigation.All results have been normalized to 413C = -25% vs PDB. The determinations yield values of the reservoir effect in agreement with earlier results obtained from shells and mammals. The final results are discussed in light of previous variations of 14C content in the atmosphere. Using a smoother curve, the reservoir effect is slightly smaller than was hitherto believed.An event thought to be of cosmic origin caused the count rate of both proportional and Geiger counters to increase significantly around December 4, 1978. The correction for this has been studied. The statistics for background, oxalic acid, and unknown samples, measured repeatedly after this correction, were as good as usual.

No abstract

W F Libby's new dating method from the 1940s, based on experience in physics and chemistry, opened possibilities to check and revise chronologies built on other principles than radioactive decay. Libby's method initially implied collaboration with archaeologists to demonstrate that it worked but also with physicists to improve the technique to measure low β– activities. Chemists, geophysicists, botanists, physiologists, statisticians, and other researchers have contributed to a prosperous interdisciplinary development. Some pitfalls were not recognized from the beginning, although issues such as contamination problems were foreseen by Libby. Pretreatment of samples was discussed very early by de Vries and collaborators, among others. This subject has not yet been abandoned. Closely related to pretreatment is the choice of fraction to be dated and chemicals to be used, especially for accelerator mass spectrometry (AMS) measurements. Calibration against tree rings and comparison with dates obtained using other methods as well as intercomparison projects are partly history but still very actual. The impact by man and climate is also studied since the early days of the method. Also, the carbon cycle has been of great interest. The tools for measurements and statistical analysis have been improved during these first 3 or 4 decades, allowing interpretations not possible earlier. δ13C determinations are mostly very important and useful, but sometimes they have been misleading in discussions of the origin of carbon, especially for human tissues—the metabolism was not yet fully understood. The history and development of the method can only be illustrated by selected examples in a survey like this.

No abstract

The following list covers the samples measured at the Uppsala radiocarbon laboratory during 1957, when the measurements started, and 1958. Two samples of sediments have been excluded, as the origin of the material was doubtful.