This paper deals with initiation and propagation processes of streamer discharges in water subjected to high-speed repetitive voltage pulse. The 50%-duty repetitive pulses were produced by the reciprocal traveling wave in a pulse forming cable which was connected with a point-plane electrode gap in a water-cell. Laue plot of time lag distributions for the streamer initiation indicated that the initiation probability during the second pulse application became much higher than that during the first pulse application. We concluded that the change in space charges distribution due to internal field during the rest-time after the first pulse enhanced the streamer initiation probability at the second pulse application. Temporal development in the positive streamers during the repetitive pulse application was observed using a gated image intensifier. When the pulse was relatively high, the streamer discharges started the propagation at the first pulse and then the discharge channel became long step by step at the subsequent pulse applications. It was also found that the periodical emission due to excitation of OH radicals was detected for a long period after the development of the streamer discharge in a spectroscopic measurement.
This paper describes experimental results of NO removal using barrier discharges produced by a reciprocal pulse generator. When a coaxial cable is charged and then grounded at one end of the cable without any resistance, a reciprocal traveling voltage pulse is repeatedly applied to a barrier-type reactor at the opposite end with a change in its polarity. 50% streamer initiation voltage for the reciprocal pulse generator was much smaller than that with the self-matched pulse generator having a matching resistance. The reason for the low initiation voltage in the reciprocal pulse was that space charges which accumulated on the barrier surface during cable charging had an effect on field enhancement in the reactor after the first polarity reversal. High speed photographs of discharge light produced by the reciprocal pulse showed that the voltage oscillation caused by one switching induced alternate propagation of positive and negative streamers with a very high frequency. In measurements of NO concentration, the reciprocal pulse generator gave a better performance for NO removal ratio than the self-matched pulse generator even though the stored energy in the recipocal pulse generator was very low.
An anomalous discharge current flowing in the same direction as the charging current was observed in a low-density polyethylene film with evaporated silver electrodes at room temperature (25°C) after the application of a very high field above 2×108 V/m.
The discharge transient current was computer-analyzed numerically by an explicit difference method. The anomalous current was attributed to the large amount of two types of injected space charge (electrons and holes) with ohmic electrodes, and not to one type of injected space charge (electrons or holes) with blocking electrodes.
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