This study evaluated the CO2 sequestration potential with combustion ashes in the aqueous phase. The aim was to provide a cost-effective carbon sequestration method for combustion unit operators (flue gas cleaning) or biogas producers (biogas upgrading). Therefore, two separate test series were executed to identify the carbonation efficiency (CE) of bottom wood ash (1) at different mixing ratios with water in batch experiments and (2) under dynamic flow conditions. It was furthermore evaluated whether subsequent use of the carbonated wood ash for soil amendment could be possible and whether the process water could be passed into the sewage. The batch test series showed that different mixing ratios of wood ash and water had an influence on the CE. The flow series showed that the mean CE varied between approximately 14% and 17%. Thus, the ash proved to be suitable for carbonation processes. The process water was dischargeable, and the carbonated wood ash has potential for chalking, as no legal thresholds were exceeded. Therefore, wood ash carbonation could be used as a low-tech CO2 sequestration technology. Compared to existing energy consuming and cost intensive carbon capture and storage technologies, sequestration with ash could be beneficial, as it represents a low-tech approach.
This study evaluates the anaerobic digestion (AD) of the organic fraction of municipal solid waste (OFMSW) and digested sewage sludge (DSS) at lowered temperatures. AD batch tests for CH4 yield determination were carried out with DSS as inoculum between 23 and 40 °C. All results were related to organic dry matter and calculated for standard conditions (1013 hPa, 0 °C). The AD experiments at 40 °C and at 35 °C delivered specific CH4 yields of 325 ± 6 mL/g and 268 ± 27 mL/g for OFMSW alone. At lower temperatures, specific CH4 yields of 364 ± 25 mL/g (25 °C) and 172 ± 21 mL/g (23 °C) were reached. AD at 25 °C could be beneficial regarding energy input (heating costs) and energy output (CH4 yield). Plant operators could increase AD efficiencies by avoiding heating costs. The co-digestion of OFMSW together with DSS could lead to further synergies such as better exploitation of the energy potentials of DSS, but the digestate utilization could become problematic due to hygienic requirements. Efficiency potentials through lowered operating temperatures are limited. In further research, lowered process temperatures could be applied in the AD of energy crops due to large numbers of existing plants.
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