A deep machine-learning technique based on a convolutional neural network (CNN) is introduced. It has been used for the classification of powder X-ray diffraction (XRD) patterns in terms of crystal system, extinction group and space group. About 150 000 powder XRD patterns were collected and used as input for the CNN with no handcrafted engineering involved, and thereby an appropriate CNN architecture was obtained that allowed determination of the crystal system, extinction group and space group. In sharp contrast with the traditional use of powder XRD pattern analysis, the CNN never treats powder XRD patterns as a deconvoluted and discrete peak position or as intensity data, but instead the XRD patterns are regarded as nothing but a pattern similar to a picture. The CNN interprets features that humans cannot recognize in a powder XRD pattern. As a result, accuracy levels of 81.14, 83.83 and 94.99% were achieved for the space-group, extinction-group and crystal-system classifications, respectively. The well trained CNN was then used for symmetry identification of unknown novel inorganic compounds.
Complicated structures consisting of multi-layers with a multi-modal array of device components, i.e., so-called patterned multi-layers, and their corresponding circuit designs for signal readout and addressing are used to achieve a macroscale electronic skin (e-skin). In contrast to this common approach, we realized an extremely simple macroscale e-skin only by employing a single-layered piezoresistive MWCNT-PDMS composite film with neither nano-, micro-, nor macro-patterns. It is the deep machine learning that made it possible to let such a simple bulky material play the role of a smart sensory device. A deep neural network (DNN) enabled us to process electrical resistance change induced by applied pressure and thereby to instantaneously evaluate the pressure level and the exact position under pressure. The great potential of this revolutionary concept for the attainment of pressure-distribution sensing on a macroscale area could expand its use to not only e-skin applications but to other high-end applications such as touch panels, portable flexible keyboard, sign language interpreting globes, safety diagnosis of social infrastructures, and the diagnosis of motility and peristalsis disorders in the gastrointestinal tract.
An extremely simple bulk sheet made of a piezoresistive carbon nanotube (CNT)-Ecoflex composite can act as a smart keypad that is portable, disposable, and flexible enough to be carried crushed inside the pocket of a pair of trousers. Both a rigid-button-imbedded, rollable (or foldable) pad and a patterned flexible pad have been introduced for use as portable keyboards. Herein, we suggest a bare, bulk, macroscale piezoresistive sheet as a replacement for these complex devices that are achievable only through high-cost fabrication processes such as patterning-based coating, printing, deposition, and mounting. A deep-learning technique based on deep neural networks (DNN) enables this extremely simple bulk sheet to play the role of a smart keypad without the use of complicated fabrication processes. To develop this keypad, instantaneous electrical resistance change was recorded at several locations on the edge of the sheet along with the exact information on the touch position and pressure for a huge number of random touches. The recorded data were used for training a DNN model that could eventually act as a brain for a simple sheet-type keypad. This simple sheet-type keypad worked perfectly and outperformed all of the existing portable keypads in terms of functionality, flexibility, disposability, and cost.
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