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Hierarchical porous mixed metal oxide/graphene two‐dimensional nanostructures, providing an extra active position for lithium storage, represent a hopeful platform for next‐generation anode materials. Herein, we report a facile approach to synthesize micro‐/mesoporous zinc–manganese oxide/graphene (Zn‐Mn‐O/G) hybrids with a specific surface area of 227.6 m2 g−1 in a water/ethanol mixed solvent. Owing to the micro‐/mesoporous structure, large specific area, and strongly coupled effects between Zn‐Mn‐O and the graphene sheets, the hybrids deliver a high capacity of 1216 mAh g−1 at a current density of 500 mA g−1 after 100 cycles, a superior rate performance of 558 mAh g−1 at 8000 mA g−1, as well as ultralong cycle life up to 900 cycles. In addition, if performed in the temperature range of 5 to 45 °C, the Zn‐Mn‐O/G anode demonstrates specific capacities between 748 and 1245 mAh g−1 after 100 cycles.

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