The availability of photon states with well-defined temporal modes is crucial for photonic quantum technologies. Ever since the inception of generating photonic quantum states through pulse pumped spontaneous parametric processes, many exquisite efforts have been put on improving the modal purity of the photon states to achieve single-mode operation. However, because the nonlinear interaction and linear dispersion are often mixed in parametric processes, limited successes have been achieved so far only at some specific wavelengths with sophisticated design. In this paper, we resort to a different approach by exploiting an active filtering mechanism originated from interference fringe of nonlinear interferometer. The nonlinear interferometer is realized in a sequential array of nonlinear medium, with a gap in between made of a linear dispersive medium, in which the precise modal control is realized without influencing the phase matching of the parametric process. As a proof-of-principle demonstration of the capability, we present a photon pairs source using a two-stage nonlinear interferometer formed by two identical nonlinear fibers with a standard single mode fiber in between. The results show that spectrally correlated two-photon state via four wave mixing in a single piece nonlinear fiber is modified into factorable state and heralded single-photons with high modal purity and high heralding efficiency are achievable. This novel quantum interferometric method, which can improve the quality of the photon states in almost all the aspects such as modal purity, heralding efficiency, and flexibility in wavelength selection, is proved to be effective and easy to realize.

Multiphoton quantum interference is the underlying principle for optical quantum information processing protocols. Indistinguishability is the key to quantum interference. Therefore, the success of many protocols in optical quantum information processing relies on the availability of photon states with a well-defined spatial and temporal mode. Photons in single spatial mode can be obtained from nonlinear processes in single-mode waveguides. For the temporal mode, the common approach is to engineer the nonlinear processes so as to achieve the required spectral properties for the generated photons. But, this approach is complicated because the spectral properties and the nonlinear interaction are often intertwined through phase-matching condition. In this paper, we study a different approach that separates the spectral control from nonlinear interaction, leading to versatile and precise engineering of the spectral properties of nonlinear parametric processes. The approach is based on an SU(1,1) nonlinear interferometer with a pulsed pump and a controllable linear spectral phase shift for precise engineering. We systematically analyze the important figures of merit such as modal purity and heralding efficiency in characterizing a photon state and use this analysis to investigate the feasibility of this interferometric approach. Specifically, we analyze in detail the requirement on the spectral phase engineering to optimize the figures of merit and apply numerical simulations to the nonlinear four-wave mixing process in dispersion-shifted fibers with a standard single-mode fiber as the phase control medium. Both modal purity and efficiency are improved simultaneously with this technique. Furthermore, a multistage nonlinear interferometer is proposed and shown to achieve more precise state engineering for near-ideal single-mode operation and near-unity efficiency. We also extend the study to the case of high pump power when the high gain is achieved in the four-wave mixing process for the spectral engineering of quantum entanglement in continuous variables. Our investigation provides an approach for precisely tailoring the spectral property of quantum light sources, especially, photon pairs can be engineered to simultaneously possess the features of high purity, high collection efficiency, high brightness, and high flexibility in wavelength and bandwidth selection.

We experimentally study a fiber-based three-stage nonlinear interferometer and demonstrate its application in generating heralded single photons with high efficiency and purity by spectral engineering. We obtain a heralding efficiency of 90% at a brightness of 0.039 photons/pulse. The purity of the source is checked by two-photon Hong-Ou-Mandel interference with a visibility of 95 ± 6% (after correcting Raman scattering and multi-pair events). Our investigation indicates that the heralded source of single photons produced by the three-stage nonlinear interferometer has the advantages of high purity, high heralding efficiency, high brightness, and flexibility in wavelength and bandwidth selection.

Few-mode fibers (FMFs) have been recently employed in classical optical communication to increase the data transmission capacity. Here we explore the capability of employing FMF for long distance quantum communication. We experimentally distribute photon pairs in the forms of time-bin and polarization entanglement over a 1-km-long FMF. We find the time-bin entangled photon pairs maintain their high degree of entanglement, no matter what type of spatial modes they are distributed in. For the polarization entangled photon pairs, however, the degree of entanglement is maintained when photon pairs are distributed in LP 01 mode but significantly declines when photon pairs are distributed in LP 11 mode due to a mode coupling effect in LP 11 mode group. We propose and test a remedy to recover the high degree of entanglement. Our study shows, when FMFs are employed as quantum channels, selection of spatial channels and degrees of freedom of entanglement should be carefully considered.